Angewandte Chemie - International Edition, volume 60, issue 40, pages 21979-21987
Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts
Weiwei Guo
1, 2
,
Shoujie Liu
3
,
Xingxing Tan
1, 2
,
RUIZHI WU
1, 2
,
Xupeng Yan
1, 2
,
Chunjun Chen
1
,
Qinggong Zhu
1
,
Li-Rong Zheng
4
,
Jingyuan Ma
5
,
Jian Zhang
4
,
YUYING HUANG
5
,
Xiaofu Sun
1, 2
,
Buxing Han
1, 2, 6, 7
3
Chemistry and Chemical Engineering of Guangdong Laboratory Shantou 515063 China
|
6
Physical Science Laboratory Huairou National Comprehensive Science Center Beijing 101400 China
|
Publication type: Journal Article
Publication date: 2021-08-27
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 16.6
ISSN: 14337851, 15213773
General Chemistry
Catalysis
Abstract
We have prepared atomically dispersed Sn catalysts on defective CuO for CO2 electroreduction to methanol. The Faradaic efficiency of methanol could reach 88.6 % with a current density of 67.0 mA cm−2. The catalyst was beneficial for CO2 activation via decreasing the energy barrier of *COOH dissociation to form *CO. The *CO was then bound to the Cu species for further reduction, leading to high selectivity toward methanol.
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Guo W. et al. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.
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Guo W., Liu S., Tan X., WU R., Yan X., Chen C., Zhu Q., Zheng L., Ma J., Zhang J., HUANG Y., Sun X., Han B. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.
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TY - JOUR
DO - 10.1002/anie.202108635
UR - https://doi.org/10.1002/anie.202108635
TI - Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts
T2 - Angewandte Chemie - International Edition
AU - Tan, Xingxing
AU - WU, RUIZHI
AU - Yan, Xupeng
AU - HUANG, YUYING
AU - Han, Buxing
AU - Guo, Weiwei
AU - Liu, Shoujie
AU - Chen, Chunjun
AU - Zhu, Qinggong
AU - Zheng, Li-Rong
AU - Ma, Jingyuan
AU - Zhang, Jian
AU - Sun, Xiaofu
PY - 2021
DA - 2021/08/27
PB - Wiley
SP - 21979-21987
IS - 40
VL - 60
SN - 1433-7851
SN - 1521-3773
ER -
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BibTex
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@article{2021_Guo,
author = {Xingxing Tan and RUIZHI WU and Xupeng Yan and YUYING HUANG and Buxing Han and Weiwei Guo and Shoujie Liu and Chunjun Chen and Qinggong Zhu and Li-Rong Zheng and Jingyuan Ma and Jian Zhang and Xiaofu Sun},
title = {Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {aug},
url = {https://doi.org/10.1002/anie.202108635},
number = {40},
pages = {21979--21987},
doi = {10.1002/anie.202108635}
}
Cite this
MLA
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Guo, Weiwei, et al. “Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts.” Angewandte Chemie - International Edition, vol. 60, no. 40, Aug. 2021, pp. 21979-21987. https://doi.org/10.1002/anie.202108635.