volume 60 issue 40 pages 21979-21987

Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts

Weiwei Guo 1, 2
Shoujie Liu 3
Xingxing Tan 1, 2
RUIZHI WU 1, 2
Xupeng Yan 1, 2
Chunjun Chen 1
Qinggong Zhu 1
Li-Rong Zheng 4
Jingyuan Ma 5
Jian Zhang 4
YUYING HUANG 5
Xiaofu Sun 1, 2
Buxing Han 1, 2, 6, 7
Publication typeJournal Article
Publication date2021-08-27
scimago Q1
wos Q1
SJR5.550
CiteScore27.6
Impact factor16.9
ISSN14337851, 15213773
General Chemistry
Catalysis
Abstract
We have prepared atomically dispersed Sn catalysts on defective CuO for CO2 electroreduction to methanol. The Faradaic efficiency of methanol could reach 88.6 % with a current density of 67.0 mA cm−2. The catalyst was beneficial for CO2 activation via decreasing the energy barrier of *COOH dissociation to form *CO. The *CO was then bound to the Cu species for further reduction, leading to high selectivity toward methanol.
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GOST Copy
Guo W. et al. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.
GOST all authors (up to 50) Copy
Guo W., Liu S., Tan X., WU R., Yan X., Chen C., Zhu Q., Zheng L., Ma J., Zhang J., HUANG Y., Sun X., Han B. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1002/anie.202108635
UR - https://doi.org/10.1002/anie.202108635
TI - Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts
T2 - Angewandte Chemie - International Edition
AU - Guo, Weiwei
AU - Liu, Shoujie
AU - Tan, Xingxing
AU - WU, RUIZHI
AU - Yan, Xupeng
AU - Chen, Chunjun
AU - Zhu, Qinggong
AU - Zheng, Li-Rong
AU - Ma, Jingyuan
AU - Zhang, Jian
AU - HUANG, YUYING
AU - Sun, Xiaofu
AU - Han, Buxing
PY - 2021
DA - 2021/08/27
PB - Wiley
SP - 21979-21987
IS - 40
VL - 60
PMID - 34346160
SN - 1433-7851
SN - 1521-3773
ER -
BibTex |
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BibTex (up to 50 authors) Copy
@article{2021_Guo,
author = {Weiwei Guo and Shoujie Liu and Xingxing Tan and RUIZHI WU and Xupeng Yan and Chunjun Chen and Qinggong Zhu and Li-Rong Zheng and Jingyuan Ma and Jian Zhang and YUYING HUANG and Xiaofu Sun and Buxing Han},
title = {Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {aug},
url = {https://doi.org/10.1002/anie.202108635},
number = {40},
pages = {21979--21987},
doi = {10.1002/anie.202108635}
}
MLA
Cite this
MLA Copy
Guo, Weiwei, et al. “Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts.” Angewandte Chemie - International Edition, vol. 60, no. 40, Aug. 2021, pp. 21979-21987. https://doi.org/10.1002/anie.202108635.