Angewandte Chemie - International Edition

, том 60 , издание 40 , страницы 21979-21987

Highly Efficient CO ₂ Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts

Weiwei Guo ^{1, 2}

Shoujie Liu ³

Xingxing Tan ^{1, 2}

RUIZHI WU ^{1, 2}

Xupeng Yan ^{1, 2}

Chunjun Chen ¹

Qinggong Zhu ¹

Li-Rong Zheng ⁴

Jingyuan Ma ⁵

Jian Zhang ⁴

YUYING HUANG ⁵

Xiaofu Sun ^{1, 2}

Buxing Han ^{1, 2, 6, 7}

Скрыть аффилиации авторов Показать аффилиации авторов: 7 аффилиаций

Beijing National Laboratory for Molecular Sciences CAS Key Laboratory of Colloid and Interface and Thermodynamics CAS Research/Education Center for Excellence in Molecular Sciences Institute of Chemistry Chinese Academy of Sciences Zhongguancun North First Street 2 Beijing 100190 China

Институт химии Китайской академии наук

Пекинская национальная лаборатория молекулярных наук

School of Chemistry and Chemical Engineering University of Chinese Academy of Sciences Yuquan Road, ShijingshanDistrict Beijing 100049 China |

Chemistry and Chemical Engineering of Guangdong Laboratory Shantou 515063 China |

⁴

Institute of High Energy Physics Chinese Academy of Sciences Beijing 100049 China |

⁵

Shanghai Synchrotron Radiation Facility, Zhangjiang Laboratory (SSRF, ZJLab) Shanghai Advanced Research Institute Chinese Academy of Sciences Shanghai 201204 China |

⁶

Physical Science Laboratory Huairou National Comprehensive Science Center Beijing 101400 China |

⁷

Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular Engineering East China Normal University Shanghai 200062 China |

Тип публикации: Journal Article

Дата публикации: 2021-08-27

Wiley

Angewandte Chemie - International Edition

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wos Q1

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SJR: 5.550

CiteScore: 27.6

Impact factor: 16.9

ISSN: 14337851, 15213773

DOI: 10.1002/anie.202108635

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PubMed ID: 34346160

General Chemistry

Catalysis

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We have prepared atomically dispersed Sn catalysts on defective CuO for CO2 electroreduction to methanol. The Faradaic efficiency of methanol could reach 88.6 % with a current density of 67.0 mA cm−2. The catalyst was beneficial for CO2 activation via decreasing the energy barrier of *COOH dissociation to form *CO. The *CO was then bound to the Cu species for further reduction, leading to high selectivity toward methanol.

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Guo W. et al. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.

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Guo W., Liu S., Tan X., WU R., Yan X., Chen C., Zhu Q., Zheng L., Ma J., Zhang J., HUANG Y., Sun X., Han B. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.

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TY - JOUR

DO - 10.1002/anie.202108635

UR - https://doi.org/10.1002/anie.202108635

TI - Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts

T2 - Angewandte Chemie - International Edition

AU - Guo, Weiwei

AU - Liu, Shoujie

AU - Tan, Xingxing

AU - WU, RUIZHI

AU - Yan, Xupeng

AU - Chen, Chunjun

AU - Zhu, Qinggong

AU - Zheng, Li-Rong

AU - Ma, Jingyuan

AU - Zhang, Jian

AU - HUANG, YUYING

AU - Sun, Xiaofu

AU - Han, Buxing

PY - 2021

DA - 2021/08/27

PB - Wiley

SP - 21979-21987

IS - 40

VL - 60

PMID - 34346160

SN - 1433-7851

SN - 1521-3773

ER -

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@article{2021_Guo,

author = {Weiwei Guo and Shoujie Liu and Xingxing Tan and RUIZHI WU and Xupeng Yan and Chunjun Chen and Qinggong Zhu and Li-Rong Zheng and Jingyuan Ma and Jian Zhang and YUYING HUANG and Xiaofu Sun and Buxing Han},

title = {Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts},

journal = {Angewandte Chemie - International Edition},

year = {2021},

volume = {60},

publisher = {Wiley},

month = {aug},

url = {https://doi.org/10.1002/anie.202108635},

number = {40},

pages = {21979--21987},

doi = {10.1002/anie.202108635}

}

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Guo, Weiwei, et al. “Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts.” Angewandte Chemie - International Edition, vol. 60, no. 40, Aug. 2021, pp. 21979-21987. https://doi.org/10.1002/anie.202108635.

Издатель

Wiley

Журнал

Angewandte Chemie - International Edition

scimago Q1

wos Q1

БС1

SJR

5.550

CiteScore

27.6

Impact factor

16.9

ISSN

14337851 (Print)

15213773 (Electronic)