Angewandte Chemie - International Edition

, том 60 , издание 40 , страницы 21979-21987

Highly Efficient CO ₂ Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts

Тип публикации: Journal Article

Дата публикации: 2021-08-27

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Angewandte Chemie - International Edition

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SJR: 5.495

CiteScore: 27.6

Impact factor: 16.9

ISSN: 14337851, 15213773

DOI: 10.1002/anie.202108635

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PubMed ID: 34346160

General Chemistry

Catalysis

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We have prepared atomically dispersed Sn catalysts on defective CuO for CO2 electroreduction to methanol. The Faradaic efficiency of methanol could reach 88.6 % with a current density of 67.0 mA cm−2. The catalyst was beneficial for CO2 activation via decreasing the energy barrier of *COOH dissociation to form *CO. The *CO was then bound to the Cu species for further reduction, leading to high selectivity toward methanol.

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Guo W. et al. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.

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Guo W., Liu S., Tan X., WU R., Yan X., Chen C., Zhu Q., Zheng L., Ma J., Zhang J., HUANG Y., Sun X., Han B. Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 40. pp. 21979-21987.

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TY - JOUR

DO - 10.1002/anie.202108635

UR - https://doi.org/10.1002/anie.202108635

TI - Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts

T2 - Angewandte Chemie - International Edition

AU - Guo, Weiwei

AU - Liu, Shoujie

AU - Tan, Xingxing

AU - WU, RUIZHI

AU - Yan, Xupeng

AU - Chen, Chunjun

AU - Zhu, Qinggong

AU - Zheng, Li-Rong

AU - Ma, Jingyuan

AU - Zhang, Jian

AU - HUANG, YUYING

AU - Sun, Xiaofu

AU - Han, Buxing

PY - 2021

DA - 2021/08/27

PB - Wiley

SP - 21979-21987

IS - 40

VL - 60

PMID - 34346160

SN - 1433-7851

SN - 1521-3773

ER -

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@article{2021_Guo,

author = {Weiwei Guo and Shoujie Liu and Xingxing Tan and RUIZHI WU and Xupeng Yan and Chunjun Chen and Qinggong Zhu and Li-Rong Zheng and Jingyuan Ma and Jian Zhang and YUYING HUANG and Xiaofu Sun and Buxing Han},

title = {Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts},

journal = {Angewandte Chemie - International Edition},

year = {2021},

volume = {60},

publisher = {Wiley},

month = {aug},

url = {https://doi.org/10.1002/anie.202108635},

number = {40},

pages = {21979--21987},

doi = {10.1002/anie.202108635}

}

MLA

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Guo, Weiwei, et al. “Highly Efficient CO 2 Electroreduction to Methanol through Atomically Dispersed Sn Coupled with Defective CuO Catalysts.” Angewandte Chemie - International Edition, vol. 60, no. 40, Aug. 2021, pp. 21979-21987. https://doi.org/10.1002/anie.202108635.

Издатель

Wiley

Журнал

Angewandte Chemie - International Edition

SCImago Q1

Tоп 10% SCImago

WOS Q1

БС1