Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides
2
UCB Biopharma 1420 Braine-l'Alleud Belgium
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3
Medicinal Chemistry Janssen Research & Development 2340 Beerse Belgium
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Publication type: Journal Article
Publication date: 2021-11-02
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
34558788
General Chemistry
Catalysis
Abstract
The unusual stereochemical feature of certain sulfonimidamides, in which tautomeric forms are also enantiomeric, has been exploited to develop a catalytic enantioselective synthesis of alkylated sulfonimidamides. The reactions proceed through a prochiral anionic intermediate to deliver enantiomerically enriched products. A double-alkylated, cinchona alkaloid-derived catalyst is used as a phase-transfer catalyst.
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45
Total citations:
45
Citations from 2025:
23
(51.11%)
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Tilby M. J. et al. Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 49. pp. 25680-25687.
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Tilby M. J., Dewez D. F., Hall A., Martínez Lamenca C., Willis M. J. Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 49. pp. 25680-25687.
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TY - JOUR
DO - 10.1002/anie.202109160
UR - https://doi.org/10.1002/anie.202109160
TI - Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides
T2 - Angewandte Chemie - International Edition
AU - Tilby, Michael J
AU - Dewez, Damien F
AU - Hall, Adrian
AU - Martínez Lamenca, Carolina
AU - Willis, M. J.
PY - 2021
DA - 2021/11/02
PB - Wiley
SP - 25680-25687
IS - 49
VL - 60
PMID - 34558788
SN - 1433-7851
SN - 1521-3773
ER -
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BibTex (up to 50 authors)
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@article{2021_Tilby,
author = {Michael J Tilby and Damien F Dewez and Adrian Hall and Carolina Martínez Lamenca and M. J. Willis},
title = {Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/anie.202109160},
number = {49},
pages = {25680--25687},
doi = {10.1002/anie.202109160}
}
Cite this
MLA
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Tilby, Michael J., et al. “Exploiting Configurational Lability in Aza‐Sulfur Compounds for the Organocatalytic Enantioselective Synthesis of Sulfonimidamides.” Angewandte Chemie - International Edition, vol. 60, no. 49, Nov. 2021, pp. 25680-25687. https://doi.org/10.1002/anie.202109160.