Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework
Publication type: Journal Article
Publication date: 2021-11-17
scimago Q1
wos Q1
SJR: 5.550
CiteScore: 27.6
Impact factor: 16.9
ISSN: 14337851, 15213773
PubMed ID:
34676638
General Chemistry
Catalysis
Abstract
Stimuli-responsive materials that can be reversibly switched by light are of immense interest. Among them, photo-responsive spin crossover (SCO) complexes have great promises to combine the photoactive inputs with multifaceted outputs into switchable materials and devices. However, the reversible control the spin-state change by photochromic guests is still challenging. Herein, we report an unprecedented guest-driven light-induced spin change (GD-LISC) in a Hofmann-type metal-organic framework (MOF), [Fe(bpn){Ag(CN)2 }2 ]⋅azobenzene. (1, bpn=1,4-bis(4-pyridyl)naphthalene). The reversible trans-cis photoisomerization of azobenzene guest upon UV/Vis irradiation in the solid-state results in the remarkable magnetic changes in a wide temperature range of 10-180 K. This finding not only establishes a new switching mechanism for SCO complexes, but also paves the way toward the development of new generation of photo-responsive magnetic materials.
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64
Total citations:
64
Citations from 2025:
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(15.63%)
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GOST
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Xie K. P. et al. Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 52. pp. 27144-27150.
GOST all authors (up to 50)
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Xie K. P., Ruan Z. Yu., Lyu B. H., Wang Y., Zhang X., Huang G., Chen Y., Ni Z. P., Tong M. Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework // Angewandte Chemie - International Edition. 2021. Vol. 60. No. 52. pp. 27144-27150.
Cite this
RIS
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TY - JOUR
DO - 10.1002/anie.202113294
UR - https://doi.org/10.1002/anie.202113294
TI - Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework
T2 - Angewandte Chemie - International Edition
AU - Xie, Kai Ping
AU - Ruan, Ze Yu
AU - Lyu, Bang Heng
AU - Wang, Yueming
AU - Zhang, Xue-Wen
AU - Huang, Guo-Zhang
AU - Chen, Yancong
AU - Ni, Zhao Ping
AU - Tong, Mingliang
PY - 2021
DA - 2021/11/17
PB - Wiley
SP - 27144-27150
IS - 52
VL - 60
PMID - 34676638
SN - 1433-7851
SN - 1521-3773
ER -
Cite this
BibTex (up to 50 authors)
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@article{2021_Xie,
author = {Kai Ping Xie and Ze Yu Ruan and Bang Heng Lyu and Yueming Wang and Xue-Wen Zhang and Guo-Zhang Huang and Yancong Chen and Zhao Ping Ni and Mingliang Tong},
title = {Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework},
journal = {Angewandte Chemie - International Edition},
year = {2021},
volume = {60},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/anie.202113294},
number = {52},
pages = {27144--27150},
doi = {10.1002/anie.202113294}
}
Cite this
MLA
Copy
Xie, Kai Ping, et al. “Guest‐Driven Light‐Induced Spin Change in an Azobenzene Loaded Metal–Organic Framework.” Angewandte Chemie - International Edition, vol. 60, no. 52, Nov. 2021, pp. 27144-27150. https://doi.org/10.1002/anie.202113294.