Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons
Publication type: Journal Article
Publication date: 2019-10-23
scimago Q2
wos Q2
SJR: 0.751
CiteScore: 5.9
Impact factor: 3.3
ISSN: 18614728, 1861471X
PubMed ID:
31550070
General Chemistry
Organic Chemistry
Biochemistry
Abstract
The dihalomethanes CH2X2 (X=Cl, Br, I) were co‐crystallized with the isocyanide complexes trans‐[MXM2(CNC6H4‐4‐XC)2] (M=Pd, Pt; XM=Br, I; XC=F, Cl, Br) to give an extended series comprising 15 X‐ray structures of isostructural adducts featuring 1D metal‐involving hexagon‐like arrays. In these structures, CH2X2 behave as bent bifunctional XB/XB‐donating building blocks, whereas trans‐[MXM2(CNC6H4‐4‐XC)2] act as a linear XB/XB acceptors. Results of DFT calculations indicate that all XCH2–X⋅⋅⋅XM–M contacts are typical noncovalent interactions with estimated strengths in the range of 1.3–3.2 kcal mol−1. A CCDC search reveals that hexagon‐like arrays are rather common but previously overlooked structural motives for adducts of trans‐bis(halide) complexes and halomethanes.
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Metrics
60
Total citations:
60
Citations from 2024:
16
(26.67%)
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GOST
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Kashina M. V. et al. Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons // Chemistry - An Asian Journal. 2019. Vol. 14. No. 21. pp. 3915-3920.
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Kashina M. V., Kinzhalov M. A., Smirnov M. S., Ivanov D. M., Novikov A. S., Kukushkin V. Y. Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons // Chemistry - An Asian Journal. 2019. Vol. 14. No. 21. pp. 3915-3920.
Cite this
RIS
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TY - JOUR
DO - 10.1002/asia.201901127
UR - https://onlinelibrary.wiley.com/doi/10.1002/asia.201901127
TI - Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons
T2 - Chemistry - An Asian Journal
AU - Kashina, Maria V
AU - Kinzhalov, M. A.
AU - Smirnov, Mikhail S.
AU - Ivanov, Daniil M
AU - Novikov, Alexander S.
AU - Kukushkin, Vadim Yu.
PY - 2019
DA - 2019/10/23
PB - Wiley
SP - 3915-3920
IS - 21
VL - 14
PMID - 31550070
SN - 1861-4728
SN - 1861-471X
ER -
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BibTex (up to 50 authors)
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@article{2019_Kashina,
author = {Maria V Kashina and M. A. Kinzhalov and Mikhail S. Smirnov and Daniil M Ivanov and Alexander S. Novikov and Vadim Yu. Kukushkin},
title = {Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons},
journal = {Chemistry - An Asian Journal},
year = {2019},
volume = {14},
publisher = {Wiley},
month = {oct},
url = {https://onlinelibrary.wiley.com/doi/10.1002/asia.201901127},
number = {21},
pages = {3915--3920},
doi = {10.1002/asia.201901127}
}
Cite this
MLA
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Kashina, Maria V., et al. “Dihalomethanes as Bent Bifunctional XB/XB-Donating Building Blocks for Construction of Metal-involving Halogen Bonded Hexagons.” Chemistry - An Asian Journal, vol. 14, no. 21, Oct. 2019, pp. 3915-3920. https://onlinelibrary.wiley.com/doi/10.1002/asia.201901127.