Atom-economic approach to the synthesis of α-(hetero)aryl substituted furan derivatives from biomass.
Publication type: Journal Article
Publication date: 2021-12-09
scimago Q2
wos Q2
SJR: 0.751
CiteScore: 5.9
Impact factor: 3.3
ISSN: 18614728, 1861471X
PubMed ID:
34807522
General Chemistry
Organic Chemistry
Biochemistry
Abstract
An atom-economic ring construction approach to the synthesis of α-(hetero)arylfurans based on renewable furanic platform chemicals has been developed. Corresponding compounds have been prepared in good to excellent yields via [2+2+2] and [4+2] cycloaddition reactions using metal-catalyzed or photoredox protocols. Easily available HMF-based 2-hydroxymethyl-5-ethynylfuran and 2-hydroxymethyl-5-cyanofuran were used as starting materials. A synthetic route with an improved carbon economy factor has been implemented to achieve sustainability aim. The possible application of arylfurans as molecular conductors has been investigated by DFT calculations, which revealed excellent charge transfer properties. As a future perspective, integration of biomass processing strategy into manufacturing of molecular electronics was pointed out to achieve the aim of sustainability.
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8
Total citations:
8
Citations from 2024:
4
(50%)
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Romashov L. V. et al. Atom-economic approach to the synthesis of α-(hetero)aryl substituted furan derivatives from biomass. // Chemistry - An Asian Journal. 2021. Vol. 17. No. 1.
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Romashov L. V., Kozlov K. S., Skorobogatko M. K., Kostyukovich A. Y., Ananikov V. P. Atom-economic approach to the synthesis of α-(hetero)aryl substituted furan derivatives from biomass. // Chemistry - An Asian Journal. 2021. Vol. 17. No. 1.
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TY - JOUR
DO - 10.1002/asia.202101227
UR - https://doi.org/10.1002/asia.202101227
TI - Atom-economic approach to the synthesis of α-(hetero)aryl substituted furan derivatives from biomass.
T2 - Chemistry - An Asian Journal
AU - Romashov, Leonid V.
AU - Kozlov, Kirill S.
AU - Skorobogatko, Matvey K
AU - Kostyukovich, Alexander Y
AU - Ananikov, Valentine P.
PY - 2021
DA - 2021/12/09
PB - Wiley
IS - 1
VL - 17
PMID - 34807522
SN - 1861-4728
SN - 1861-471X
ER -
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@article{2021_Romashov,
author = {Leonid V. Romashov and Kirill S. Kozlov and Matvey K Skorobogatko and Alexander Y Kostyukovich and Valentine P. Ananikov},
title = {Atom-economic approach to the synthesis of α-(hetero)aryl substituted furan derivatives from biomass.},
journal = {Chemistry - An Asian Journal},
year = {2021},
volume = {17},
publisher = {Wiley},
month = {dec},
url = {https://doi.org/10.1002/asia.202101227},
number = {1},
doi = {10.1002/asia.202101227}
}
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