Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation
Lidiya Kibis
1
,
Olga Podyacheva
2
,
E.M Slavinskaya
2
,
Abdelwahab H Hassan
3, 4
,
Silke Hampel
4
,
Albrecht Leonhardt
4
,
Z. R. Ismagilov
2
,
Aleksandr S. Noskov
2
,
Publication type: Journal Article
Publication date: 2014-05-21
scimago Q1
wos Q2
SJR: 0.941
CiteScore: 6.1
Impact factor: 3.9
ISSN: 18673880, 18673899
Catalysis
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The oxidation of CO over Pd nanoparticles supported on carbon nanofibers (CNFs) and N‐doped carbon nanofibers (N‐CNFs) has been studied. Investigation by scanning transmission electron microscopy together with electron energy‐loss spectroscopy revealed that Pd nanoparticles are located on the N‐CNFs surface patches that have a high concentration of N atoms. The N‐doping of CNFs was shown to change the electric conductivity of N‐CNFs and redox properties of Pd, which thus determines the self‐oscillatory behavior of the catalysts during CO oxidation, the type of oscillations, and the conditions of their generation. Mechanisms that underlie the effect of N in N‐CNFs on the electronic state of Pd as well as the occurrence of two types of oscillation mechanisms—the known redox mechanism and the mechanism related to Pd intercalation into graphene layers—are discussed.
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GOST
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Kibis L. et al. Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation // ChemCatChem. 2014. Vol. 6. No. 7. pp. 2115-2128.
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Kibis L., Podyacheva O., Slavinskaya E., Zaikovskii V. I., Hassan A. H., Hampel S., Leonhardt A., Ismagilov Z. R., Noskov A. S., Boronin A. I. Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation // ChemCatChem. 2014. Vol. 6. No. 7. pp. 2115-2128.
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TY - JOUR
DO - 10.1002/cctc.201402108
UR - https://doi.org/10.1002/cctc.201402108
TI - Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation
T2 - ChemCatChem
AU - Kibis, Lidiya
AU - Podyacheva, Olga
AU - Slavinskaya, E.M
AU - Zaikovskii, Vladimir I
AU - Hassan, Abdelwahab H
AU - Hampel, Silke
AU - Leonhardt, Albrecht
AU - Ismagilov, Z. R.
AU - Noskov, Aleksandr S.
AU - Boronin, Andrey I
PY - 2014
DA - 2014/05/21
PB - Wiley
SP - 2115-2128
IS - 7
VL - 6
SN - 1867-3880
SN - 1867-3899
ER -
Cite this
BibTex (up to 50 authors)
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@article{2014_Kibis,
author = {Lidiya Kibis and Olga Podyacheva and E.M Slavinskaya and Vladimir I Zaikovskii and Abdelwahab H Hassan and Silke Hampel and Albrecht Leonhardt and Z. R. Ismagilov and Aleksandr S. Noskov and Andrey I Boronin},
title = {Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation},
journal = {ChemCatChem},
year = {2014},
volume = {6},
publisher = {Wiley},
month = {may},
url = {https://doi.org/10.1002/cctc.201402108},
number = {7},
pages = {2115--2128},
doi = {10.1002/cctc.201402108}
}
Cite this
MLA
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Kibis, Lidiya, et al. “Palladium Nanoparticles Supported on Nitrogen‐Doped Carbon Nanofibers: Synthesis, Microstructure, Catalytic Properties, and Self‐Sustained Oscillation Phenomena in Carbon Monoxide Oxidation.” ChemCatChem, vol. 6, no. 7, May. 2014, pp. 2115-2128. https://doi.org/10.1002/cctc.201402108.