Open Access

ChemElectroChem, volume 5, issue 7, pages 1064-1072

Effects of Anion Identity and Concentration on Electrochemical Reduction of CO ₂

Joaquin Resasco ^{1, 2}

Yanwei Lum ^{2, 3}

Ezra Clark ^{1, 2}

José A. Zamora Zeledón ^{1, 2}

Alexis T. Bell ^{1, 2}

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Department of Chemical Engineering University of California Berkeley, CA 94720 |

Joint Center for Artificial Photosynthesis, Material Science Division Lawrence Berkeley National Laboratory Berkeley, CA 94720 |

Department of Materials Science and Engineering University of California Berkeley, CA 94720 |

Publication type: Journal Article

Publication date: 2018-02-12

Wiley

Journal: ChemElectroChem

Quartile SCImago

Quartile WOS

Impact factor: 4

ISSN: 21960216, 21960216

DOI: 10.1002/celc.201701316

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Catalysis

Electrochemistry

Abstract

Author(s): Resasco, J; Lum, Y; Clark, E; Zeledon, JZ; Bell, AT | Abstract: The electrochemical reduction of CO2 is known to be influenced by the concentration and identity of the anionic species in the electrolyte; however, a full understanding of this phenomenon has not been developed. Here, we present the results of experimental and computational studies aimed at understanding the role of electrolyte anions on the reduction of CO2 over Cu surfaces. Experimental studies were performed to show the effects of bicarbonate buffer concentration and the composition of other buffering anions on the partial currents of the major products formed by reduction of CO2 over Cu. It was demonstrated that the composition and concentration of electrolyte anions has relatively little effect on the formation of CO, HCOO−, C2H4, and CH3CH2OH, but has a significant effect on the formation of H2 and CH4. Continuum modeling was used to assess the effects of buffering anions on the pH at the electrode surface. The influence of pH on the activity of Cu for producing H2 and CH4 was also considered. Changes in the pH near the electrode surface were insufficient to explain the differences in activity and selectivity observed with changes in anion buffering capacity observed for the formation of H2 and CH4. Therefore, it is proposed that these differences are the result of the ability of buffering anions to donate hydrogen directly to the electrode surface and in competition with water. The effectiveness of buffering anions to serve as hydrogen donors is found to increase with decreasing pKa of the buffering anion.

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	2 4 6 8 10 12 14 16 18
ACS Catalysis	ACS Catalysis, 17, 10.18% ACS Catalysis 17 publications, 10.18%
ACS Energy Letters	ACS Energy Letters, 9, 5.39% ACS Energy Letters 9 publications, 5.39%
Journal of the American Chemical Society	Journal of the American Chemical Society, 8, 4.79% Journal of the American Chemical Society 8 publications, 4.79%
Electrochimica Acta	Electrochimica Acta, 6, 3.59% Electrochimica Acta 6 publications, 3.59%
Nature Catalysis	Nature Catalysis, 5, 2.99% Nature Catalysis 5 publications, 2.99%
ChemElectroChem	ChemElectroChem, 4, 2.4% ChemElectroChem 4 publications, 2.4%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 4, 2.4% Journal of Physical Chemistry C 4 publications, 2.4%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 2.4% ACS applied materials & interfaces 4 publications, 2.4%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 4, 2.4% Journal of Materials Chemistry A 4 publications, 2.4%
Energy and Environmental Science	Energy and Environmental Science, 4, 2.4% Energy and Environmental Science 4 publications, 2.4%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 3, 1.8% Journal of the Electrochemical Society 3 publications, 1.8%
Nature Communications	Nature Communications, 3, 1.8% Nature Communications 3 publications, 1.8%
Chem Catalysis	Chem Catalysis, 3, 1.8% Chem Catalysis 3 publications, 1.8%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 3, 1.8% Applied Catalysis B: Environmental 3 publications, 1.8%
Advanced Functional Materials	Advanced Functional Materials, 3, 1.8% Advanced Functional Materials 3 publications, 1.8%
ChemSusChem	ChemSusChem, 3, 1.8% ChemSusChem 3 publications, 1.8%
Chemical Reviews	Chemical Reviews, 3, 1.8% Chemical Reviews 3 publications, 1.8%
ACS Applied Energy Materials	ACS Applied Energy Materials, 3, 1.8% ACS Applied Energy Materials 3 publications, 1.8%
Accounts of Chemical Research	Accounts of Chemical Research, 3, 1.8% Accounts of Chemical Research 3 publications, 1.8%
Chemical Science	Chemical Science, 3, 1.8% Chemical Science 3 publications, 1.8%
Nanoscale	Nanoscale, 3, 1.8% Nanoscale 3 publications, 1.8%
Transactions of Tianjin University	Transactions of Tianjin University, 2, 1.2% Transactions of Tianjin University 2 publications, 1.2%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.2% Chemical Engineering Journal 2 publications, 1.2%
Applied Surface Science	Applied Surface Science, 2, 1.2% Applied Surface Science 2 publications, 1.2%
iScience	iScience, 2, 1.2% iScience 2 publications, 1.2%
Journal of Catalysis	Journal of Catalysis, 2, 1.2% Journal of Catalysis 2 publications, 1.2%
Advanced Materials	Advanced Materials, 2, 1.2% Advanced Materials 2 publications, 1.2%
Chemical Society Reviews	Chemical Society Reviews, 2, 1.2% Chemical Society Reviews 2 publications, 1.2%
Electrochemical Science Advances	Electrochemical Science Advances, 2, 1.2% Electrochemical Science Advances 2 publications, 1.2%
	2 4 6 8 10 12 14 16 18

Citations by publishers

	10 20 30 40 50 60 70
American Chemical Society (ACS)	American Chemical Society (ACS), 61, 36.53% American Chemical Society (ACS) 61 publications, 36.53%
Elsevier	Elsevier, 33, 19.76% Elsevier 33 publications, 19.76%
Wiley	Wiley, 24, 14.37% Wiley 24 publications, 14.37%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 21, 12.57% Royal Society of Chemistry (RSC) 21 publications, 12.57%
Springer Nature	Springer Nature, 15, 8.98% Springer Nature 15 publications, 8.98%
The Electrochemical Society	The Electrochemical Society, 3, 1.8% The Electrochemical Society 3 publications, 1.8%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 2, 1.2% Multidisciplinary Digital Publishing Institute (MDPI) 2 publications, 1.2%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.6% Frontiers Media S.A. 1 publication, 0.6%
Tianjin Daxue/Tianjin University	Tianjin Daxue/Tianjin University, 1, 0.6% Tianjin Daxue/Tianjin University 1 publication, 0.6%
Cambridge University Press	Cambridge University Press, 1, 0.6% Cambridge University Press 1 publication, 0.6%
IOP Publishing	IOP Publishing, 1, 0.6% IOP Publishing 1 publication, 0.6%
Chemical Industry Press	Chemical Industry Press, 1, 0.6% Chemical Industry Press 1 publication, 0.6%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.6% American Association for the Advancement of Science (AAAS) 1 publication, 0.6%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.6% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.6%
	10 20 30 40 50 60 70

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Resasco J. et al. Effects of Anion Identity and Concentration on Electrochemical Reduction of CO 2 // ChemElectroChem. 2018. Vol. 5. No. 7. pp. 1064-1072.

GOST all authors (up to 50) Copy

Resasco J., Lum Y., Clark E., Zamora Zeledón J. A., Bell A. T. Effects of Anion Identity and Concentration on Electrochemical Reduction of CO 2 // ChemElectroChem. 2018. Vol. 5. No. 7. pp. 1064-1072.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1002/celc.201701316

UR - https://doi.org/10.1002/celc.201701316

TI - Effects of Anion Identity and Concentration on Electrochemical Reduction of CO 2

T2 - ChemElectroChem

AU - Resasco, Joaquin

AU - Lum, Yanwei

AU - Clark, Ezra

AU - Zamora Zeledón, José A.

AU - Bell, Alexis T.

PY - 2018

DA - 2018/02/12 00:00:00

PB - Wiley

SP - 1064-1072

IS - 7

VL - 5

SN - 2196-0216

ER -

BibTex |

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BibTex Copy

@article{2018_Resasco,

author = {Joaquin Resasco and Yanwei Lum and Ezra Clark and José A. Zamora Zeledón and Alexis T. Bell},

title = {Effects of Anion Identity and Concentration on Electrochemical Reduction of CO 2},

journal = {ChemElectroChem},

year = {2018},

volume = {5},

publisher = {Wiley},

month = {feb},

url = {https://doi.org/10.1002/celc.201701316},

number = {7},

pages = {1064--1072},

doi = {10.1002/celc.201701316}

}

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Resasco, Joaquin, et al. “Effects of Anion Identity and Concentration on Electrochemical Reduction of CO 2.” ChemElectroChem, vol. 5, no. 7, Feb. 2018, pp. 1064-1072. https://doi.org/10.1002/celc.201701316.

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Wiley

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ChemElectroChem

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Quartile WOS

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21960216 (Electronic)
21960216 (Print)