volume 14 issue 8 pages 2420-2434

Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond

Publication typeJournal Article
Publication date2008-03-07
scimago Q1
wos Q2
SJR0.981
CiteScore6.7
Impact factor3.7
ISSN09476539, 15213765
General Chemistry
Catalysis
Organic Chemistry
Abstract
We have developed two new catalytic systems based on Ni and Pd complexes to solve the challenging problem of dialkyldichalcogenide (Alk2E2; E=S, Se) addition to alkynes. A comparative study of two catalytic systems-Ni/PMe2Ph and Pd/PCy2Ph-has revealed that the Ni catalyst is superior with respect to high catalytic activity and more general scope relative to the Pd system. A novel synthetic methodology was developed for the preparation of (Z)-bis(alkylthio)alkenes and (Z)-bis(alkylseleno)alkenes from terminal alkynes with excellent stereoselectivity and high yields.
Found 
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Ananikov V. P. et al. Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond // Chemistry - A European Journal. 2008. Vol. 14. No. 8. pp. 2420-2434.
GOST all authors (up to 50) Copy
Ananikov V. P., Gayduk K. A., Beletskaya I. P., Khrustalev V. N., Antipin M. Y. Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond // Chemistry - A European Journal. 2008. Vol. 14. No. 8. pp. 2420-2434.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1002/chem.200701278
UR - https://doi.org/10.1002/chem.200701278
TI - Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond
T2 - Chemistry - A European Journal
AU - Ananikov, Valentine P.
AU - Gayduk, Konstantin A
AU - Beletskaya, Irina P.
AU - Khrustalev, Victor N.
AU - Antipin, Mikhail Yu.
PY - 2008
DA - 2008/03/07
PB - Wiley
SP - 2420-2434
IS - 8
VL - 14
PMID - 18213556
SN - 0947-6539
SN - 1521-3765
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2008_Ananikov,
author = {Valentine P. Ananikov and Konstantin A Gayduk and Irina P. Beletskaya and Victor N. Khrustalev and Mikhail Yu. Antipin},
title = {Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond},
journal = {Chemistry - A European Journal},
year = {2008},
volume = {14},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/chem.200701278},
number = {8},
pages = {2420--2434},
doi = {10.1002/chem.200701278}
}
MLA
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MLA Copy
Ananikov, Valentine P., et al. “Remarkable ligand effect in Ni- And Pd-catalyzed bisthiolation and bisselenation of terminal alkynes: Solving the problem of stereoselective dialkyldichalcogenide addition to the C≡C bond.” Chemistry - A European Journal, vol. 14, no. 8, Mar. 2008, pp. 2420-2434. https://doi.org/10.1002/chem.200701278.