Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes
Rua B Alnoman
1
,
Sandra Rihn
1
,
Daniel C Oconnor
1
,
Fiona A. Black
1
,
Bernard Costello
2
,
Paul G. Waddell
1
,
William Clegg
1
,
Robert D. Peacock
3
,
Wouter Herrebout
4, 5, 6
,
Julian G Knight
1
,
M. J. Hall
1
2
Applied Photophysics Ltd., 21 Mole Business Park, Leatherhead, Surrey KT22 7BA (UK)
|
4
DEPARTMENT OF CHEMISTRY
6
Groenenborgerlaan 171 2020 Antwerp Belgium
|
Publication type: Journal Article
Publication date: 2015-11-30
scimago Q1
wos Q2
SJR: 0.981
CiteScore: 6.7
Impact factor: 3.7
ISSN: 09476539, 15213765
PubMed ID:
26555772
General Chemistry
Catalysis
Organic Chemistry
Abstract
Helically chiral N,N,O,O-boron chelated dipyrromethenes showed solution-phase circularly polarized luminescence (CPL) in the red region of the visible spectrum (λem (max) from 621 to 663 nm). The parent dipyrromethene is desymmetrised through O chelation of boron by the 3,5-ortho-phenolic substituents, inducing a helical chirality in the fluorophore. The combination of high luminescence dissymmetry factors (|glum | up to 4.7 ×10(-3) ) and fluorescence quantum yields (ΦF up to 0.73) gave exceptionally efficient circularly polarized red emission from these simple small organic fluorophores, enabling future application in CPL-based bioimaging.
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Citations from 2024:
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(15.15%)
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Alnoman R. B. et al. Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes // Chemistry - A European Journal. 2015. Vol. 22. No. 1. pp. 93-96.
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Alnoman R. B., Rihn S., Oconnor D. C., Black F. A., Costello B., Waddell P. G., Clegg W., Peacock R. D., Herrebout W., Knight J. G., Hall M. J. Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes // Chemistry - A European Journal. 2015. Vol. 22. No. 1. pp. 93-96.
Cite this
RIS
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TY - JOUR
DO - 10.1002/chem.201504484
UR - https://doi.org/10.1002/chem.201504484
TI - Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes
T2 - Chemistry - A European Journal
AU - Alnoman, Rua B
AU - Rihn, Sandra
AU - Oconnor, Daniel C
AU - Black, Fiona A.
AU - Costello, Bernard
AU - Waddell, Paul G.
AU - Clegg, William
AU - Peacock, Robert D.
AU - Herrebout, Wouter
AU - Knight, Julian G
AU - Hall, M. J.
PY - 2015
DA - 2015/11/30
PB - Wiley
SP - 93-96
IS - 1
VL - 22
PMID - 26555772
SN - 0947-6539
SN - 1521-3765
ER -
Cite this
BibTex (up to 50 authors)
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@article{2015_Alnoman,
author = {Rua B Alnoman and Sandra Rihn and Daniel C Oconnor and Fiona A. Black and Bernard Costello and Paul G. Waddell and William Clegg and Robert D. Peacock and Wouter Herrebout and Julian G Knight and M. J. Hall},
title = {Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes},
journal = {Chemistry - A European Journal},
year = {2015},
volume = {22},
publisher = {Wiley},
month = {nov},
url = {https://doi.org/10.1002/chem.201504484},
number = {1},
pages = {93--96},
doi = {10.1002/chem.201504484}
}
Cite this
MLA
Copy
Alnoman, Rua B., et al. “Circularly Polarized Luminescence from Helically Chiral N ,N ,O ,O -Boron-Chelated Dipyrromethenes.” Chemistry - A European Journal, vol. 22, no. 1, Nov. 2015, pp. 93-96. https://doi.org/10.1002/chem.201504484.