Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles
Publication type: Journal Article
Publication date: 2021-03-04
scimago Q1
wos Q2
SJR: 0.981
CiteScore: 6.7
Impact factor: 3.7
ISSN: 09476539, 15213765
PubMed ID:
33427338
General Chemistry
Catalysis
Organic Chemistry
Abstract
The zirconium catalyzed hydroaminoalkylation of alkenes with N-aryl- and sterically demanding N-alkyl-α-arylated secondary amines by using commercially available Zr(NMe2 )4 is reported. N-phenyl- and N-isopropylbenzylamine are used as amine substrates to establish the alkene substrate scope. Exclusively linear products are obtained in the presence of bulky vinylsilanes. Challenging α-heteroarylated amines and functionalized alkene substrates are compatible with this easy to use catalyst, affording a new disconnection strategy for the atom- and step-economic preparation of selectively substituted saturated α-arylated heterocycles.
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17
Total citations:
17
Citations from 2024:
4
(23.52%)
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Koperniku A., Schafer L. L. Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles // Chemistry - A European Journal. 2021. Vol. 27. No. 20. pp. 6334-6339.
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Koperniku A., Schafer L. L. Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles // Chemistry - A European Journal. 2021. Vol. 27. No. 20. pp. 6334-6339.
Cite this
RIS
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TY - JOUR
DO - 10.1002/chem.202100014
UR - https://doi.org/10.1002/chem.202100014
TI - Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles
T2 - Chemistry - A European Journal
AU - Koperniku, Ana
AU - Schafer, Laurel L
PY - 2021
DA - 2021/03/04
PB - Wiley
SP - 6334-6339
IS - 20
VL - 27
PMID - 33427338
SN - 0947-6539
SN - 1521-3765
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2021_Koperniku,
author = {Ana Koperniku and Laurel L Schafer},
title = {Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles},
journal = {Chemistry - A European Journal},
year = {2021},
volume = {27},
publisher = {Wiley},
month = {mar},
url = {https://doi.org/10.1002/chem.202100014},
number = {20},
pages = {6334--6339},
doi = {10.1002/chem.202100014}
}
Cite this
MLA
Copy
Koperniku, Ana, et al. “Zirconium Catalyzed Hydroaminoalkylation for the Synthesis of α‐Arylated Amines and N‐Heterocycles.” Chemistry - A European Journal, vol. 27, no. 20, Mar. 2021, pp. 6334-6339. https://doi.org/10.1002/chem.202100014.