Mechanochemical Synthesis of Non‐Solvated Dialkylalumanyl Anion and XPS Characterization of Al(I) and Al(II) Species
Тип публикации: Journal Article
Дата публикации: 2023-12-11
scimago Q1
wos Q2
БС1
SJR: 0.981
CiteScore: 6.7
Impact factor: 3.7
ISSN: 09476539, 15213765
PubMed ID:
38018466
General Chemistry
Catalysis
Organic Chemistry
Краткое описание
A non‐solvated alkyl‐substituted Al(I) anion dimer was synthesized by a reduction of haloalumane precursor using a mechanochemical method. The crystallographic and theoretical analysis revealed its structure and electronic properties. Experimental XPS analysis of the Al(I) anions with reference compounds revealed the lower Al 2p binding energy corresponds to the lower oxidation state of Al species. It should be emphasized that the experimentally obtained XPS binding energies were reproduced by delta SCF calculations and were linearly correlated with NPA charges and 2p orbital energies.
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Kurumada S. et al. Mechanochemical Synthesis of Non‐Solvated Dialkylalumanyl Anion and XPS Characterization of Al(I) and Al(II) Species // Chemistry - A European Journal. 2023. Vol. 30. No. 7.
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Kurumada S., Yamanashi R., Sugita K., Kubota K., Ito H., Ikemoto S., Chen C., Moriyama T., Muratsugu S., Tada M., Koitaya T., OZAKI T., Yamashita M. Mechanochemical Synthesis of Non‐Solvated Dialkylalumanyl Anion and XPS Characterization of Al(I) and Al(II) Species // Chemistry - A European Journal. 2023. Vol. 30. No. 7.
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TY - JOUR
DO - 10.1002/chem.202303073
UR - https://doi.org/10.1002/chem.202303073
TI - Mechanochemical Synthesis of Non‐Solvated Dialkylalumanyl Anion and XPS Characterization of Al(I) and Al(II) Species
T2 - Chemistry - A European Journal
AU - Kurumada, Satoshi
AU - Yamanashi, Ryotaro
AU - Sugita, Kengo
AU - Kubota, Koji
AU - Ito, Hajime
AU - Ikemoto, Satoru
AU - Chen, Chaoqi
AU - Moriyama, Takumi
AU - Muratsugu, Satoshi
AU - Tada, Mizuki
AU - Koitaya, Takanori
AU - OZAKI, TAISUKE
AU - Yamashita, Makoto
PY - 2023
DA - 2023/12/11
PB - Wiley
IS - 7
VL - 30
PMID - 38018466
SN - 0947-6539
SN - 1521-3765
ER -
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@article{2023_Kurumada,
author = {Satoshi Kurumada and Ryotaro Yamanashi and Kengo Sugita and Koji Kubota and Hajime Ito and Satoru Ikemoto and Chaoqi Chen and Takumi Moriyama and Satoshi Muratsugu and Mizuki Tada and Takanori Koitaya and TAISUKE OZAKI and Makoto Yamashita},
title = {Mechanochemical Synthesis of Non‐Solvated Dialkylalumanyl Anion and XPS Characterization of Al(I) and Al(II) Species},
journal = {Chemistry - A European Journal},
year = {2023},
volume = {30},
publisher = {Wiley},
month = {dec},
url = {https://doi.org/10.1002/chem.202303073},
number = {7},
doi = {10.1002/chem.202303073}
}