ChemSusChem, volume 8, issue 13, pages 2154-2175

Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives.

Julian Kalhoff ¹

Gebrekidan Gebresilassie Eshetu ²

Dominic Bresser ^{2, 3}

Stefano Passerini ²

Hide authors affiliations Show authors affiliations: 3 affiliations

Institute of Physical Chemistry and MEET Battery Research Center, University of Münster, Corrensstr. 28/30 & 46, 48149 Münster (Germany) |

Karlsruhe Institute of Technology (KIT), PO Box 3640, 76021 Karlsruhe (Germany) |

Institut Nanosciences et Cryogénie/Structure et Propriétés d'Architectures Moléculaires/Polymères Conducteurs Ionique (INAC/SPRAM/PCI), CEA-Grenoble, UMR-5819, CEA-CNRS-UJF, 17 Rue de Martyrs, 38054 Grenoble, Cedex 9 (France) |

Publication type: Journal Article

Publication date: 2015-06-15

Wiley

Journal: ChemSusChem

Quartile SCImago

Quartile WOS

Impact factor: 8.4

ISSN: 18645631, 1864564X

DOI: 10.1002/cssc.201500284

Copy DOI

General Chemical Engineering

General Materials Science

General Energy

Environmental Chemistry

Abstract

Lithium-ion batteries are becoming increasingly important for electrifying the modern transportation system and, thus, hold the promise to enable sustainable mobility in the future. However, their large-scale application is hindered by severe safety concerns when the cells are exposed to mechanical, thermal, or electrical abuse conditions. These safety issues are intrinsically related to their superior energy density, combined with the (present) utilization of highly volatile and flammable organic-solvent-based electrolytes. Herein, state-of-the-art electrolyte systems and potential alternatives are briefly surveyed, with a particular focus on their (inherent) safety characteristics. The challenges, which so far prevent the widespread replacement of organic carbonate-based electrolytes with LiPF6 as the conducting salt, are also reviewed herein. Starting from rather "facile" electrolyte modifications by (partially) replacing the organic solvent or lithium salt and/or the addition of functional electrolyte additives, conceptually new electrolyte systems, including ionic liquids, solvent-free, and/or gelled polymer-based electrolytes, as well as solid-state electrolytes, are also considered. Indeed, the opportunities for designing new electrolytes appear to be almost infinite, which certainly complicates strict classification of such systems and a fundamental understanding of their properties. Nevertheless, these innumerable opportunities also provide a great chance of developing highly functionalized, new electrolyte systems, which may overcome the afore-mentioned safety concerns, while also offering enhanced mechanical, thermal, physicochemical, and electrochemical performance.

By date By citations

Top-30

Citations by journals

	5 10 15 20 25 30 35 40
Journal of Power Sources	Journal of Power Sources, 40, 5.99% Journal of Power Sources 40 publications, 5.99%
Electrochimica Acta	Electrochimica Acta, 35, 5.24% Electrochimica Acta 35 publications, 5.24%
ACS applied materials & interfaces	ACS applied materials & interfaces, 31, 4.64% ACS applied materials & interfaces 31 publications, 4.64%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 22, 3.29% Journal of the Electrochemical Society 22 publications, 3.29%
Advanced Energy Materials	Advanced Energy Materials, 21, 3.14% Advanced Energy Materials 21 publications, 3.14%
Energy Storage Materials	Energy Storage Materials, 18, 2.69% Energy Storage Materials 18 publications, 2.69%
ChemSusChem	ChemSusChem, 17, 2.54% ChemSusChem 17 publications, 2.54%
Batteries & Supercaps	Batteries & Supercaps, 15, 2.25% Batteries & Supercaps 15 publications, 2.25%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 15, 2.25% Journal of Materials Chemistry A 15 publications, 2.25%
Chemical Engineering Journal	Chemical Engineering Journal, 11, 1.65% Chemical Engineering Journal 11 publications, 1.65%
ACS Applied Energy Materials	ACS Applied Energy Materials, 11, 1.65% ACS Applied Energy Materials 11 publications, 1.65%
Batteries	Batteries, 10, 1.5% Batteries 10 publications, 1.5%
ChemElectroChem	ChemElectroChem, 10, 1.5% ChemElectroChem 10 publications, 1.5%
Advanced Functional Materials	Advanced Functional Materials, 9, 1.35% Advanced Functional Materials 9 publications, 1.35%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 9, 1.35% Journal of Physical Chemistry C 9 publications, 1.35%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 8, 1.2% Angewandte Chemie - International Edition 8 publications, 1.2%
Macromolecules	Macromolecules, 8, 1.2% Macromolecules 8 publications, 1.2%
Solid State Ionics	Solid State Ionics, 8, 1.2% Solid State Ionics 8 publications, 1.2%
Energy Technology	Energy Technology, 8, 1.2% Energy Technology 8 publications, 1.2%
Angewandte Chemie	Angewandte Chemie, 8, 1.2% Angewandte Chemie 8 publications, 1.2%
Journal of Physical Chemistry B	Journal of Physical Chemistry B, 8, 1.2% Journal of Physical Chemistry B 8 publications, 1.2%
Energy and Environmental Science	Energy and Environmental Science, 8, 1.2% Energy and Environmental Science 8 publications, 1.2%
RSC Advances	RSC Advances, 7, 1.05% RSC Advances 7 publications, 1.05%
Chemistry of Materials	Chemistry of Materials, 6, 0.9% Chemistry of Materials 6 publications, 0.9%
Small	Small, 6, 0.9% Small 6 publications, 0.9%
Journal of Molecular Liquids	Journal of Molecular Liquids, 6, 0.9% Journal of Molecular Liquids 6 publications, 0.9%
Nano Energy	Nano Energy, 6, 0.9% Nano Energy 6 publications, 0.9%
Advanced Materials	Advanced Materials, 6, 0.9% Advanced Materials 6 publications, 0.9%
Chemical Communications	Chemical Communications, 6, 0.9% Chemical Communications 6 publications, 0.9%
	5 10 15 20 25 30 35 40

Citations by publishers

	50 100 150 200 250
Elsevier	Elsevier, 206, 30.84% Elsevier 206 publications, 30.84%
Wiley	Wiley, 149, 22.31% Wiley 149 publications, 22.31%
American Chemical Society (ACS)	American Chemical Society (ACS), 110, 16.47% American Chemical Society (ACS) 110 publications, 16.47%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 76, 11.38% Royal Society of Chemistry (RSC) 76 publications, 11.38%
Springer Nature	Springer Nature, 33, 4.94% Springer Nature 33 publications, 4.94%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 26, 3.89% Multidisciplinary Digital Publishing Institute (MDPI) 26 publications, 3.89%
The Electrochemical Society	The Electrochemical Society, 22, 3.29% The Electrochemical Society 22 publications, 3.29%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 6, 0.9% American Institute of Physics (AIP) 6 publications, 0.9%
Frontiers Media S.A.	Frontiers Media S.A., 5, 0.75% Frontiers Media S.A. 5 publications, 0.75%
IOP Publishing	IOP Publishing, 4, 0.6% IOP Publishing 4 publications, 0.6%
Taylor & Francis	Taylor & Francis, 4, 0.6% Taylor & Francis 4 publications, 0.6%
The Korean Electrochemical Society	The Korean Electrochemical Society, 2, 0.3% The Korean Electrochemical Society 2 publications, 0.3%
OAE Publishing Inc.	OAE Publishing Inc., 2, 0.3% OAE Publishing Inc. 2 publications, 0.3%
American Physical Society (APS)	American Physical Society (APS), 1, 0.15% American Physical Society (APS) 1 publication, 0.15%
The Chemical Society of Japan	The Chemical Society of Japan, 1, 0.15% The Chemical Society of Japan 1 publication, 0.15%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 1, 0.15% The Electrochemical Society of Japan 1 publication, 0.15%
Pleiades Publishing	Pleiades Publishing, 1, 0.15% Pleiades Publishing 1 publication, 0.15%
Walter de Gruyter	Walter de Gruyter, 1, 0.15% Walter de Gruyter 1 publication, 0.15%
Society of Fiber Science and Technology	Society of Fiber Science and Technology, 1, 0.15% Society of Fiber Science and Technology 1 publication, 0.15%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.15% American Association for the Advancement of Science (AAAS) 1 publication, 0.15%
Centre for Evaluation in Education and Science (CEON/CEES)	Centre for Evaluation in Education and Science (CEON/CEES), 1, 0.15% Centre for Evaluation in Education and Science (CEON/CEES) 1 publication, 0.15%
SAE International	SAE International, 1, 0.15% SAE International 1 publication, 0.15%
Oxford University Press	Oxford University Press, 1, 0.15% Oxford University Press 1 publication, 0.15%
American Society of Civil Engineers (ASCE)	American Society of Civil Engineers (ASCE), 1, 0.15% American Society of Civil Engineers (ASCE) 1 publication, 0.15%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.15% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.15%
	50 100 150 200 250

We do not take into account publications without a DOI.
Statistics recalculated only for publications connected to researchers, organizations and labs registered on the platform.
Statistics recalculated weekly.

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Kalhoff J. et al. Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives. // ChemSusChem. 2015. Vol. 8. No. 13. pp. 2154-2175.

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Kalhoff J., Eshetu G. G., Bresser D., Passerini S. Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives. // ChemSusChem. 2015. Vol. 8. No. 13. pp. 2154-2175.

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TY - JOUR

DO - 10.1002/cssc.201500284

UR - https://doi.org/10.1002/cssc.201500284

TI - Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives.

T2 - ChemSusChem

AU - Kalhoff, Julian

AU - Eshetu, Gebrekidan Gebresilassie

AU - Bresser, Dominic

AU - Passerini, Stefano

PY - 2015

DA - 2015/06/15 00:00:00

PB - Wiley

SP - 2154-2175

IS - 13

VL - 8

SN - 1864-5631

SN - 1864-564X

ER -

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@article{2015_Kalhoff,

author = {Julian Kalhoff and Gebrekidan Gebresilassie Eshetu and Dominic Bresser and Stefano Passerini},

title = {Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives.},

journal = {ChemSusChem},

year = {2015},

volume = {8},

publisher = {Wiley},

month = {jun},

url = {https://doi.org/10.1002/cssc.201500284},

number = {13},

pages = {2154--2175},

doi = {10.1002/cssc.201500284}

}

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Kalhoff, Julian, et al. “Safer Electrolytes for Lithium-Ion Batteries: State of the Art and Perspectives..” ChemSusChem, vol. 8, no. 13, Jun. 2015, pp. 2154-2175. https://doi.org/10.1002/cssc.201500284.

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Wiley

Journal

ChemSusChem

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8.4

ISSN

18645631 (Print)
1864564X (Electronic)