Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)]
Publication type: Journal Article
Publication date: 2017-08-28
scimago Q2
wos Q3
SJR: 0.459
CiteScore: 3.9
Impact factor: 2.0
ISSN: 14341948, 10990682
Inorganic Chemistry
Abstract
The interaction of the mixed hydrido–tetrahydridoborate ruthenium(II) complex [(Triphos)RuH(η-BH4)] [1; Triphos = κ-P-CH3C(CH2CH2PPh2)3] with alcohols of variable acidic strength [MeOH, FCH2CH2OH (MFE), CF3CH2OH (TFE), (CF3)2CHOH (HFIP), and (CF3)3COH (PFTB)] was the subject of a combined computational (DFT) and spectroscopic (VT FTIR, NMR) study. The experimental spectra suggests that RuH···HO bond formation precedes the protonation of 1, and H2 evolution leads to the loss of boron and the formation of the dimetal-
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Golub I. et al. Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)] // European Journal of Inorganic Chemistry. 2017. Vol. 2017. No. 38-39. pp. 4673-4682.
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Golub I., Filippov O. A., Belkova N. V., Gutsul E. I., epstein L. M., Rossin A., Peruzzini M., Shubina E. S. Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)] // European Journal of Inorganic Chemistry. 2017. Vol. 2017. No. 38-39. pp. 4673-4682.
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RIS
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TY - JOUR
DO - 10.1002/ejic.201700624
UR - https://doi.org/10.1002/ejic.201700624
TI - Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)]
T2 - European Journal of Inorganic Chemistry
AU - Golub, Igor
AU - Filippov, Oleg A.
AU - Belkova, Natalia V
AU - Gutsul, Eugenii I
AU - epstein, Lina M.
AU - Rossin, Andrea
AU - Peruzzini, Maurizio
AU - Shubina, Elena S.
PY - 2017
DA - 2017/08/28
PB - Wiley
SP - 4673-4682
IS - 38-39
VL - 2017
SN - 1434-1948
SN - 1099-0682
ER -
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BibTex (up to 50 authors)
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@article{2017_Golub,
author = {Igor Golub and Oleg A. Filippov and Natalia V Belkova and Eugenii I Gutsul and Lina M. epstein and Andrea Rossin and Maurizio Peruzzini and Elena S. Shubina},
title = {Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)]},
journal = {European Journal of Inorganic Chemistry},
year = {2017},
volume = {2017},
publisher = {Wiley},
month = {aug},
url = {https://doi.org/10.1002/ejic.201700624},
number = {38-39},
pages = {4673--4682},
doi = {10.1002/ejic.201700624}
}
Cite this
MLA
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Golub, Igor, et al. “Competition between the Hydride Ligands of Two Types in Proton Transfer to [{κ3‐P‐CH3C(CH2CH2PPh2)3}RuH(η2‐BH4)].” European Journal of Inorganic Chemistry, vol. 2017, no. 38-39, Aug. 2017, pp. 4673-4682. https://doi.org/10.1002/ejic.201700624.