C1 -symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands
Тип публикации: Journal Article
Дата публикации: 2005-07-18
scimago Q2
wos Q3
БС2
SJR: 0.569
CiteScore: 4.5
Impact factor: 2.7
ISSN: 10221352, 15213935
Materials Chemistry
Organic Chemistry
Physical and Theoretical Chemistry
Condensed Matter Physics
Polymers and Plastics
Краткое описание
Summary: Sixteen C1‐symmetric zirconocene and one hafnocene complexes bearing the 2,5‐R2‐7H‐cyclopenta[1,2‐b:4,3‐b′]dithiophene ligand (R = H, Me, Et, Ph) linked to a substituted indenyl ligand have been synthesized and tested in propylene polymerization. Most of the C1‐symmetric zirconocenes of this type are highly active in propylene polymerization at low MAO/Zr ratios and produce poly(propylene)s (PP) in a broad range of isotacticity and melting points. The molecular weight and crystallinity of the PPs are strongly dependent upon the type of substituents on the indenyl moiety: PPs with Tm between 75 and 156 °C and viscosity average molecular weights between 100 000 and 400 000 have been obtained at 50–70 °C in liquid propylene.
General formula of the indenyl‐based zirconocenes. General formula of the indenyl‐based zirconocenes.
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Resconi L. et al. C1-symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands // Macromolecular Chemistry and Physics. 2005. Vol. 206. No. 14. pp. 1405-1438.
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Resconi L., Guidotti S., Camurati I., Frabetti R., Focante F., Nifant'ev I. E., Laishevtsev I. P. C1-symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands // Macromolecular Chemistry and Physics. 2005. Vol. 206. No. 14. pp. 1405-1438.
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TY - JOUR
DO - 10.1002/macp.200400533
UR - https://onlinelibrary.wiley.com/doi/10.1002/macp.200400533
TI - C1-symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands
T2 - Macromolecular Chemistry and Physics
AU - Resconi, Luigi
AU - Guidotti, Simona
AU - Camurati, Isabella
AU - Frabetti, Riccardo
AU - Focante, Francesca
AU - Nifant'ev, Ilya E.
AU - Laishevtsev, Ilya P
PY - 2005
DA - 2005/07/18
PB - Wiley
SP - 1405-1438
IS - 14
VL - 206
SN - 1022-1352
SN - 1521-3935
ER -
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@article{2005_Resconi,
author = {Luigi Resconi and Simona Guidotti and Isabella Camurati and Riccardo Frabetti and Francesca Focante and Ilya E. Nifant'ev and Ilya P Laishevtsev},
title = {C1-symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands},
journal = {Macromolecular Chemistry and Physics},
year = {2005},
volume = {206},
publisher = {Wiley},
month = {jul},
url = {https://onlinelibrary.wiley.com/doi/10.1002/macp.200400533},
number = {14},
pages = {1405--1438},
doi = {10.1002/macp.200400533}
}
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Resconi, Luigi, et al. “C1-symmetric heterocyclic zirconocenes as catalysts for propylene polymerization, 2 ansa-zirconocenes with linked dithienocyclopentadienyl-substituted indenyl ligands.” Macromolecular Chemistry and Physics, vol. 206, no. 14, Jul. 2005, pp. 1405-1438. https://onlinelibrary.wiley.com/doi/10.1002/macp.200400533.