Propellants, Explosives, Pyrotechnics, volume 46, issue 11, pages 1696-1708
Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate
Publication type: Journal Article
Publication date: 2021-09-22
Quartile SCImago
Q2
Quartile WOS
Q3
Impact factor: 1.8
ISSN: 07213115, 15214087
General Chemistry
General Chemical Engineering
Abstract
This paper deals with metal oxides/carbon black (MOs/CB) composites and their influence on the thermal decomposition of ammonium perchlorate. It is shown that the developed synthesis method can be used to form the nanosized metal oxide coating on the surface of the carbon carrier. The SEM and DLS data demonstrate that the particle size for the MOs/CB catalysts ranges from 200 to 500 nm. The XRD analysis has revealed that the bivalent copper and nickel oxides are formed on the surface of the carbon support. The DSC study on the effect of MOs/CB on the thermolysis of ammonium perchlorate shows that the MOs/CB catalysts contribute to a lowering in the peak temperatures of the low and high temperature AP decomposition stages. It has also been found that bioxide MOs / CB catalysts are more efficient in this case than monoxide catalysts. The evaluation of mass spectrometry results for the decomposition products of AP formed in the presence of carbon‐based mono‐ and bioxide catalysts makes it possible to conclude that the carbon base of metal oxide catalysts causes the low‐temperature AP decomposition to proceed deep in the composite. MOs/CB catalysts, in turn, ensure a more complete decomposition of ammonium perchlorate followed by the formation of a greater number of oxidized and reduced forms of low molecular weight composites. It has been established that, for bioxide MOs/CB catalysts, the amount of chlorine formed exceeds the corresponding value for pure AP by more than ∼4 times.
Citations by journals
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1
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AIP Conference Proceedings
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Citations by publishers
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1
2
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American Chemical Society (ACS)
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American Chemical Society (ACS)
2 publications, 33.33%
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Wiley
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Wiley
1 publication, 16.67%
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Elsevier
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Elsevier
1 publication, 16.67%
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American Institute of Physics (AIP)
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American Institute of Physics (AIP)
1 publication, 16.67%
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Pleiades Publishing
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Pleiades Publishing
1 publication, 16.67%
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1
2
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Ukhin K. O. et al. Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate // Propellants, Explosives, Pyrotechnics. 2021. Vol. 46. No. 11. pp. 1696-1708.
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Ukhin K. O., Kondrashova N. B., Valtsifer V. A., Oshchepkova T. E., Savastyanova M. A., Strelnikov V., Mokrushin I. G. Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate // Propellants, Explosives, Pyrotechnics. 2021. Vol. 46. No. 11. pp. 1696-1708.
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TY - JOUR
DO - 10.1002/prep.202100187
UR - https://doi.org/10.1002%2Fprep.202100187
TI - Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate
T2 - Propellants, Explosives, Pyrotechnics
AU - Valtsifer, Victor A
AU - Savastyanova, Maria A
AU - Oshchepkova, Tamara E
AU - Ukhin, Konstantin O
AU - Kondrashova, N B
AU - Strelnikov, Vladimir
AU - Mokrushin, Ivan G
PY - 2021
DA - 2021/09/22 00:00:00
PB - Wiley
SP - 1696-1708
IS - 11
VL - 46
SN - 0721-3115
SN - 1521-4087
ER -
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@article{2021_Ukhin,
author = {Victor A Valtsifer and Maria A Savastyanova and Tamara E Oshchepkova and Konstantin O Ukhin and N B Kondrashova and Vladimir Strelnikov and Ivan G Mokrushin},
title = {Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate},
journal = {Propellants, Explosives, Pyrotechnics},
year = {2021},
volume = {46},
publisher = {Wiley},
month = {sep},
url = {https://doi.org/10.1002%2Fprep.202100187},
number = {11},
pages = {1696--1708},
doi = {10.1002/prep.202100187}
}
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Ukhin, Konstantin O., et al. “Metal Oxides/Carbon Black (MOs/CB) Composites and Their Effect on the Thermal Decomposition of Ammonium Perchlorate.” Propellants, Explosives, Pyrotechnics, vol. 46, no. 11, Sep. 2021, pp. 1696-1708. https://doi.org/10.1002%2Fprep.202100187.