Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide
E Yu Fursova
1
,
O. V. Kuznetsova
1
,
V.I. Ovcharenko
1
,
G V Romanenko
1
,
A S Bogomyakov
1
,
M. A. Kiskin
2
,
Publication type: Journal Article
Publication date: 2007-09-01
scimago Q3
SJR: 0.305
CiteScore: 2.8
Impact factor: —
ISSN: 10665285, 15739171
General Chemistry
Abstract
A method was developed for the synthesis of mixed-metal heterospin compounds with the direct coordination of the nitroxide fragment based on the replacement of acetonitrile molecules in the heterotrinuclear complex [Co2Gd(NO3)Piv6(CH3CN)2] with nitroxide molecules. The molecular and crystal structure of the heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex [Co2Gd(NO3)Piv6(NIT-Me)2], where NIT-Me is stable nitronyl nitroxide, was established. The magnetic properties of this complex were investigated in the temperature range of 2–300 K. The coordination of nitroxide groups to CoII ions is responsible for strong exchange interactions between the unpaired electrons in the exchange clusters {>-·O-CoII}, resulting in the virtually complete spin coupling between each coordinated >N-·O group and one of the unpaired electrons of each CoII ion at temperatures below 200 K.
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Fursova E. Yu. et al. Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide // Russian Chemical Bulletin. 2007. Vol. 56. No. 9. pp. 1805-1808.
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Fursova E. Yu., Kuznetsova O. V., Ovcharenko V., Romanenko G. V., Bogomyakov A. S., Kiskin M. A., Eremenko I. L. Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide // Russian Chemical Bulletin. 2007. Vol. 56. No. 9. pp. 1805-1808.
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TY - JOUR
DO - 10.1007/s11172-007-0280-0
UR - https://doi.org/10.1007/s11172-007-0280-0
TI - Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide
T2 - Russian Chemical Bulletin
AU - Fursova, E Yu
AU - Kuznetsova, O. V.
AU - Ovcharenko, V.I.
AU - Romanenko, G V
AU - Bogomyakov, A S
AU - Kiskin, M. A.
AU - Eremenko, I. L.
PY - 2007
DA - 2007/09/01
PB - Springer Nature
SP - 1805-1808
IS - 9
VL - 56
SN - 1066-5285
SN - 1573-9171
ER -
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@article{2007_Fursova,
author = {E Yu Fursova and O. V. Kuznetsova and V.I. Ovcharenko and G V Romanenko and A S Bogomyakov and M. A. Kiskin and I. L. Eremenko},
title = {Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide},
journal = {Russian Chemical Bulletin},
year = {2007},
volume = {56},
publisher = {Springer Nature},
month = {sep},
url = {https://doi.org/10.1007/s11172-007-0280-0},
number = {9},
pages = {1805--1808},
doi = {10.1007/s11172-007-0280-0}
}
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MLA
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Fursova, E. Yu., et al. “Heterospin mixed-ligand heterotrinuclear CoII, GdIII, CoII complex with nitronyl nitroxide.” Russian Chemical Bulletin, vol. 56, no. 9, Sep. 2007, pp. 1805-1808. https://doi.org/10.1007/s11172-007-0280-0.