Product selectivity of photocatalytic CO2 reduction reactions
Publication type: Journal Article
Publication date: 2020-01-01
scimago Q1
wos Q1
SJR: 5.755
CiteScore: 35.8
Impact factor: 22.0
ISSN: 13697021, 18734103
Condensed Matter Physics
General Materials Science
Mechanical Engineering
Mechanics of Materials
Abstract
Photocatalytic carbon dioxide (CO 2 ) reduction to obtain hydrocarbon solar fuels is one of the promising strategies to solve energy crisis and complement carbon cycle. However, the low activity and poor product selectivity greatly limit its practical application. Tuning product selectivity is of great significance to improve the yield of target product and deepen the understanding of CO 2 reduction reaction mechanism. In this review, we firstly summarize the widely accepted pathways of photocatalytic CO 2 reduction reactions. Secondly, important factors affecting product selectivity are analyzed, mainly including light-excitation attributes, band structure of photocatalysts, separation of photogenerated charge carriers, adsorption/activation of reactants, surface active sites of catalytic reaction, and adsorption/desorption of intermediates. Finally, the challenges and perspectives in developing photocatalysts with high CO 2 reduction efficiency and product selectivity are presented.
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GOST
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Fu J. et al. Product selectivity of photocatalytic CO2 reduction reactions // Materials Today. 2020. Vol. 32. pp. 222-243.
GOST all authors (up to 50)
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Fu J., Jiang K., Qiu X., Yu J., Liu M. Product selectivity of photocatalytic CO2 reduction reactions // Materials Today. 2020. Vol. 32. pp. 222-243.
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RIS
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TY - JOUR
DO - 10.1016/j.mattod.2019.06.009
UR - https://doi.org/10.1016/j.mattod.2019.06.009
TI - Product selectivity of photocatalytic CO2 reduction reactions
T2 - Materials Today
AU - Fu, Junwei
AU - Jiang, Kexin
AU - Qiu, Xiaoqing
AU - Yu, Jiaguo
AU - Liu, Min
PY - 2020
DA - 2020/01/01
PB - Elsevier
SP - 222-243
VL - 32
SN - 1369-7021
SN - 1873-4103
ER -
Cite this
BibTex (up to 50 authors)
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@article{2020_Fu,
author = {Junwei Fu and Kexin Jiang and Xiaoqing Qiu and Jiaguo Yu and Min Liu},
title = {Product selectivity of photocatalytic CO2 reduction reactions},
journal = {Materials Today},
year = {2020},
volume = {32},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/j.mattod.2019.06.009},
pages = {222--243},
doi = {10.1016/j.mattod.2019.06.009}
}