Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study
Тип публикации: Journal Article
Дата публикации: 1985-01-01
scimago Q3
wos Q2
БС2
SJR: 0.426
CiteScore: 4.1
Impact factor: 2.2
ISSN: 00404020, 14645416
Organic Chemistry
Drug Discovery
Biochemistry
Краткое описание
A theoretical study has been undertaken of the relative rates and the regio- and stereo-chemistry of ring closure of a variety of alkenyl, alkenylaryl, alkenylvinyl and similar radicals. The method involves the application of MM2 force-field calculations to model transition structures for which the dimensions of the arrays of reactive centres have been obtained by MNDO-UHF techniques. The results, which generally accord with guidelines based on stereochemical considerations, show excellent qualitative and satisfactory quantitative agreement with experimental data. The method has been successfully applied to complex systems including ring closure of alkylperoxy radicals, and formation of the triquinane system by three consecutive cyclisations.
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Beckwith A. L. J., Schiesser C. H. Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study // Tetrahedron. 1985. Vol. 41. No. 19. pp. 3925-3941.
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Beckwith A. L. J., Schiesser C. H. Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study // Tetrahedron. 1985. Vol. 41. No. 19. pp. 3925-3941.
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TY - JOUR
DO - 10.1016/S0040-4020(01)97174-1
UR - https://doi.org/10.1016/S0040-4020(01)97174-1
TI - Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study
T2 - Tetrahedron
AU - Beckwith, Athelstan L. J.
AU - Schiesser, C. H.
PY - 1985
DA - 1985/01/01
PB - Elsevier
SP - 3925-3941
IS - 19
VL - 41
SN - 0040-4020
SN - 1464-5416
ER -
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@article{1985_Beckwith,
author = {Athelstan L. J. Beckwith and C. H. Schiesser},
title = {Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study},
journal = {Tetrahedron},
year = {1985},
volume = {41},
publisher = {Elsevier},
month = {jan},
url = {https://doi.org/10.1016/S0040-4020(01)97174-1},
number = {19},
pages = {3925--3941},
doi = {10.1016/S0040-4020(01)97174-1}
}
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MLA
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Beckwith, Athelstan L. J., and C. H. Schiesser. “Regio- and stereo-selectivity of alkenyl radical ring closure: A theoretical study.” Tetrahedron, vol. 41, no. 19, Jan. 1985, pp. 3925-3941. https://doi.org/10.1016/S0040-4020(01)97174-1.