, volume 448 , pages 214112

Oxo/imido heterometathesis: From molecular stoichiometric studies to well-defined heterogeneous catalysts

Pavel A Zhizhko ¹

Nikolai S Bushkov ^{2, 3}

Andrey V Pichugov ^{2, 4}

Dmitry N. Zarubin ¹

Hide authors affiliations Show authors affiliations: 4 affiliations

A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilov Str. 28, 119991 Moscow, Russia |

A. N. Nesmeyanov Institute of Organoelement Compounds, Russian Academy of Sciences, Vavilov str., 28, 119991 Moscow, Russia |

Department of Chemistry, Moscow State University, Vorob’evy Gory, 1, 119991 Moscow, Russia |

⁴

Higher Chemical College, D. Mendeleev University of Chemical Technology of Russia, Miusskaya sq., 9, 125047 Moscow, Russia |

Publication type: Journal Article

Publication date: 2021-12-01

Elsevier

Coordination Chemistry Reviews

scimago Q1

wos Q1

SJR: 4.638

CiteScore: 38.2

Impact factor: 23.5

ISSN: 00108545, 18733840

DOI: 10.1016/j.ccr.2021.214112

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Materials Chemistry

Inorganic Chemistry

Physical and Theoretical Chemistry

Abstract

• Summary of stoichiometric oxo/imido heterometathesis reactions of imido complexes. • Current progress in the development of catalytic oxo/imido heterometathesis. • SOMC towards the design of well-defined silica-supported oxo and imido complexes. Oxo/imido heterometathesis is a class of reactions that interconvert terminal transition metal oxo and imido complexes via [2 + 2] cycloaddition/cycloreversion with heteroolefins and heterocumulenes containing oxo and imino groups. In this review we summarize the literature examples of stoichiometric oxo/imido heterometathesis reactions of imido complexes with different oxo substrates and discuss the current progress in the development of catalytic oxo/imido heterometathesis. In particular, we show how application of Surface Organometallic Chemistry approach allows preparation of highly efficient oxo/imido heterometathesis catalysts based on well-defined silica-supported early transition metal oxo and imido complexes.

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Kurnakov Institute of General and Inorganic Chemistry of the Russian Academy of Sciences

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Zhizhko P. A. et al. Oxo/imido heterometathesis: From molecular stoichiometric studies to well-defined heterogeneous catalysts // Coordination Chemistry Reviews. 2021. Vol. 448. p. 214112.

GOST all authors (up to 50) Copy

Zhizhko P. A., Bushkov N. S., Pichugov A. V., Zarubin D. N. Oxo/imido heterometathesis: From molecular stoichiometric studies to well-defined heterogeneous catalysts // Coordination Chemistry Reviews. 2021. Vol. 448. p. 214112.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.ccr.2021.214112

UR - https://doi.org/10.1016/j.ccr.2021.214112

TI - Oxo/imido heterometathesis: From molecular stoichiometric studies to well-defined heterogeneous catalysts

T2 - Coordination Chemistry Reviews

AU - Zhizhko, Pavel A

AU - Bushkov, Nikolai S

AU - Pichugov, Andrey V

AU - Zarubin, Dmitry N.

PY - 2021

DA - 2021/12/01

PB - Elsevier

SP - 214112

VL - 448

SN - 0010-8545

SN - 1873-3840

ER -

BibTex

Cite this

BibTex (up to 50 authors) Copy

@article{2021_Zhizhko,

author = {Pavel A Zhizhko and Nikolai S Bushkov and Andrey V Pichugov and Dmitry N. Zarubin},

title = {Oxo/imido heterometathesis: From molecular stoichiometric studies to well-defined heterogeneous catalysts},

journal = {Coordination Chemistry Reviews},

year = {2021},

volume = {448},

publisher = {Elsevier},

month = {dec},

url = {https://doi.org/10.1016/j.ccr.2021.214112},

pages = {214112},

doi = {10.1016/j.ccr.2021.214112}

}

Publisher

Elsevier

Journal

Coordination Chemistry Reviews

scimago Q1

wos Q1

SJR

4.638

CiteScore

38.2

Impact factor

23.5

ISSN

00108545 (Print, Electronic)

18733840