Adsorption of diclofenac from aqueous solution using UiO-66-type metal-organic frameworks
Publication type: Journal Article
Publication date: 2019-03-01
scimago Q1
wos Q1
SJR: 2.696
CiteScore: 20.6
Impact factor: 13.2
ISSN: 13858947, 18733212
General Chemistry
General Chemical Engineering
Industrial and Manufacturing Engineering
Environmental Chemistry
Abstract
UiO-66 type metal organic frameworks (MOFs), including UiO-66 and UiO-66-NH2, were synthesized, characterized, and applied for the adsorptive removal of diclofenac (DCF) from aqueous solutions. The effect of synthetic conditions (e.g., different linkers and activation temperatures) and adsorptive conditions (e.g., contact time, initial concentration, temperature, and pH) on DCF removal was examined. UiO-66-NH2 showed a higher adsorption capacity than UiO-66, and the increase of activation temperature can improve the adsorption capacity of UiO-66-NH2 towards DCF. The adsorption of DCF by UiO-66-NH2 was endothermic and almost not affected by pH in the range of 4.8–7.7. The adsorption of DCF onto UiO-66 type MOFs conformed to the pseud second-order kinetic model and the Langmuir isothermal model, with adsorption capacity of 357 mg g−1 for UiO-66 and 555 mg g−1 for UiO-66-NH2. Electrostatic interaction and H-bonding possibly played a vital role for DCF adsorption. The as-prepared UiO-66 type MOFs were efficient adsorbent for DCF removal from aqueous solution.
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Zhuang S., Cheng R., Wang J. Adsorption of diclofenac from aqueous solution using UiO-66-type metal-organic frameworks // Chemical Engineering Journal. 2019. Vol. 359. pp. 354-362.
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Zhuang S., Cheng R., Wang J. Adsorption of diclofenac from aqueous solution using UiO-66-type metal-organic frameworks // Chemical Engineering Journal. 2019. Vol. 359. pp. 354-362.
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TY - JOUR
DO - 10.1016/j.cej.2018.11.150
UR - https://doi.org/10.1016/j.cej.2018.11.150
TI - Adsorption of diclofenac from aqueous solution using UiO-66-type metal-organic frameworks
T2 - Chemical Engineering Journal
AU - Zhuang, Shuting
AU - Cheng, Rong
AU - Wang, Jianlong
PY - 2019
DA - 2019/03/01
PB - Elsevier
SP - 354-362
VL - 359
SN - 1385-8947
SN - 1873-3212
ER -
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@article{2019_Zhuang,
author = {Shuting Zhuang and Rong Cheng and Jianlong Wang},
title = {Adsorption of diclofenac from aqueous solution using UiO-66-type metal-organic frameworks},
journal = {Chemical Engineering Journal},
year = {2019},
volume = {359},
publisher = {Elsevier},
month = {mar},
url = {https://doi.org/10.1016/j.cej.2018.11.150},
pages = {354--362},
doi = {10.1016/j.cej.2018.11.150}
}