Journal of Catalysis

, volume 300 , pages 251-259

Influence of extra-framework Al on the structure of the active iron sites in Fe/ZSM-35

Junying Wang ^{1, 2}

Haian Xia ³

Xiaohua Ju ³

Z FENG ³

Fengtao Fan ³

Can Li ³

Hide authors affiliations Show authors affiliations: 3 affiliations

Graduate University of Chinese Academy of Sciences, Beijing 100049 (China) |

State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian, 116023 (China). |

State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, China |

Publication type: Journal Article

Publication date: 2013-04-01

Elsevier

Journal of Catalysis

scimago Q1

wos Q1

SJR: 1.558

CiteScore: 10.9

Impact factor: 6.5

ISSN: 00219517, 10902694

DOI: 10.1016/j.jcat.2013.01.011

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Catalysis

Physical and Theoretical Chemistry

Abstract

The influence of extra-framework Al via AlCl3 deposition on the structure of the active Fe sites in Fe/ZSM35 was investigated by 29 Si MAS NMR, UV–visible diffuse reflectance spectroscopy, infrared spectroscopy, UV Raman spectroscopy, and 57 Fe Mossbauer spectroscopy combined with catalytic decomposition of N2O. It is found that high-temperature treatment considerably modifies the iron speciation. UV–visible diffuse reflectance spectra and in situ infrared spectra of NO adsorption show that a significant amount of clustered and cationic Fe species is transformed into extra-framework Fe–O–Al mixed oxide species by high-temperature treatment. UV Raman spectra and 57 Fe Mossbauer spectra suggest the generation of a

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GOST Copy

Wang J. et al. Influence of extra-framework Al on the structure of the active iron sites in Fe/ZSM-35 // Journal of Catalysis. 2013. Vol. 300. pp. 251-259.

GOST all authors (up to 50) Copy

Wang J., Xia H., Ju X., FENG Z., Fan F., Li C. Influence of extra-framework Al on the structure of the active iron sites in Fe/ZSM-35 // Journal of Catalysis. 2013. Vol. 300. pp. 251-259.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1016/j.jcat.2013.01.011

UR - https://doi.org/10.1016/j.jcat.2013.01.011

TI - Influence of extra-framework Al on the structure of the active iron sites in Fe/ZSM-35

T2 - Journal of Catalysis

AU - Wang, Junying

AU - Xia, Haian

AU - Ju, Xiaohua

AU - FENG, Z

AU - Fan, Fengtao

AU - Li, Can

PY - 2013

DA - 2013/04/01

PB - Elsevier

SP - 251-259

VL - 300

SN - 0021-9517

SN - 1090-2694

ER -

BibTex

Cite this

BibTex (up to 50 authors) Copy

@article{2013_Wang,

author = {Junying Wang and Haian Xia and Xiaohua Ju and Z FENG and Fengtao Fan and Can Li},

title = {Influence of extra-framework Al on the structure of the active iron sites in Fe/ZSM-35},

journal = {Journal of Catalysis},

year = {2013},

volume = {300},

publisher = {Elsevier},

month = {apr},

url = {https://doi.org/10.1016/j.jcat.2013.01.011},

pages = {251--259},

doi = {10.1016/j.jcat.2013.01.011}

}

Publisher

Elsevier

Journal

Journal of Catalysis

scimago Q1

wos Q1

SJR

1.558

CiteScore

10.9

Impact factor

6.5

ISSN

00219517 (Print)

10902694 (Electronic)