Polynuclear architectures with cadmium and lithium ions based on the {Li2 Cd2 (O2 CCMe3 )6 } fragment
N. V. Gogoleva
1
,
G. N. Kuznetsova
1
,
D.B. Kayumova
1
,
I. P. MALKEROVA
1
,
A. S. ALIKHANYAN
1
,
E D Barabanova
2
,
M. A. Shmelev
1
,
A.V Sidorov
1
,
Publication type: Journal Article
Publication date: 2021-02-01
scimago Q2
wos Q1
SJR: 0.629
CiteScore: 6.8
Impact factor: 3.5
ISSN: 00224596, 1095726X
Materials Chemistry
Ceramics and Composites
Electronic, Optical and Magnetic Materials
Inorganic Chemistry
Physical and Theoretical Chemistry
Condensed Matter Physics
Abstract
Abstract Molecular [Li2Cd2(L)2(Piv)6]·Solv (Piv = trimethylacetate anion, L = 2,4-lutidine (1), 2,2′-bipyrdine (2), 2,2':6′,2″-terpyridine (3),·Solv = 4MeCN (2)), chain [Li3Cd(MeCN)(THF)(Piv)5]n (4) and three-dimensional polymer [Li4Cd5(H2O)4(Piv)14]n.4H2O (5) complexes were synthesized and structurally characterized. All the new molecules contain the basic moiety {Li2Cd2(Piv)6} with the two central Li atoms connected with periphery CdII by bridging carboxylate anions. Molecular compounds 1–3 are stabilized by terminal N-donor ligands. In the chain of polymer 4 each CdII atom simultaneously belongs to the neighboring {Li2Cd2(Piv)4} moiety. The core in 5 is formed by connection the {Li2Cd2} units by the {Cd(Piv)2(H2O)4} tetradentate bridging moiety. The vaporization processes, thermodynamic characteristics of complex 2 and related dissociation products in condensed and gas phases were determined by mass spectrometry. Stability of 2 in the processes of hypothetical dissociation was additionally estimated by DFT-calculations.
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Total citations:
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Citations from 2024:
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Gogoleva N. V. et al. Polynuclear architectures with cadmium and lithium ions based on the {Li2Cd2(O2CCMe3)6} fragment // Journal of Solid State Chemistry. 2021. Vol. 294. p. 121842.
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Gogoleva N. V., Kuznetsova G. N., Kayumova D., MALKEROVA I. P., ALIKHANYAN A. S., Barabanova E. D., Shmelev M. A., Lyssenko K. A., Starikova A. A., Kiskin M. A., Sidorov A., Eremenko I. L. Polynuclear architectures with cadmium and lithium ions based on the {Li2Cd2(O2CCMe3)6} fragment // Journal of Solid State Chemistry. 2021. Vol. 294. p. 121842.
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TY - JOUR
DO - 10.1016/j.jssc.2020.121842
UR - https://doi.org/10.1016/j.jssc.2020.121842
TI - Polynuclear architectures with cadmium and lithium ions based on the {Li2Cd2(O2CCMe3)6} fragment
T2 - Journal of Solid State Chemistry
AU - Gogoleva, N. V.
AU - Kuznetsova, G. N.
AU - Kayumova, D.B.
AU - MALKEROVA, I. P.
AU - ALIKHANYAN, A. S.
AU - Barabanova, E D
AU - Shmelev, M. A.
AU - Lyssenko, Konstantin A.
AU - Starikova, Alyona A
AU - Kiskin, Mikhail A.
AU - Sidorov, A.V
AU - Eremenko, Igor L.
PY - 2021
DA - 2021/02/01
PB - Elsevier
SP - 121842
VL - 294
SN - 0022-4596
SN - 1095-726X
ER -
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BibTex (up to 50 authors)
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@article{2021_Gogoleva,
author = {N. V. Gogoleva and G. N. Kuznetsova and D.B. Kayumova and I. P. MALKEROVA and A. S. ALIKHANYAN and E D Barabanova and M. A. Shmelev and Konstantin A. Lyssenko and Alyona A Starikova and Mikhail A. Kiskin and A.V Sidorov and Igor L. Eremenko},
title = {Polynuclear architectures with cadmium and lithium ions based on the {Li2Cd2(O2CCMe3)6} fragment},
journal = {Journal of Solid State Chemistry},
year = {2021},
volume = {294},
publisher = {Elsevier},
month = {feb},
url = {https://doi.org/10.1016/j.jssc.2020.121842},
pages = {121842},
doi = {10.1016/j.jssc.2020.121842}
}