Materialia, volume 28, pages 101747
Thermokinetic study of intermetallic phase formation in an Al/Cu multilayer thin film system
Evgeny T Moiseenko
1
,
V. V. Yumashev
1, 2
,
Roman R. Altunin
1
,
Oleg V. Belousov
1, 2
,
S. M. Zharkov
1, 3
Publication type: Journal Article
Publication date: 2023-05-01
General Materials Science
Abstract
The solid-state reaction process in a multilayer thin film system (Al/Cu)50 has experimentally been studied using the methods of simultaneous thermal analysis (STA) and in situ electron diffraction. A detailed kinetic analysis of the phase formation processes during the solid-state reaction has shown that the observed solid-state transformations can be described by a statistically significant kinetic model where each stage corresponds to the reaction of the n-th order with autocatalysis. The low-temperature stage has been demonstrated to be attributable to the formation of the θ-Al2Cu phase, with the medium-temperature and high-temperature ones corresponding to the α2-AlCu3 and γ1-Al4Cu9 phases, respectively. The kinetic parameters for the formation of the phases θ-Al2Cu, α2-AlCu3 and γ1-Al4Cu9 have been determined. It has been shown that the kinetic model describing the solid-state reaction in the Al-Cu multilayer thin film system is in best agreement with the experimental data in the case of a competition between the formation stages of the α2-AlCu3 and γ1-Al4Cu9 phases.
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Moiseenko E. T. et al. Thermokinetic study of intermetallic phase formation in an Al/Cu multilayer thin film system // Materialia. 2023. Vol. 28. p. 101747.
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Moiseenko E. T., Yumashev V. V., Altunin R. R., Solovyov L. A., Volochaev M. N., Belousov O. V., Zharkov S. M. Thermokinetic study of intermetallic phase formation in an Al/Cu multilayer thin film system // Materialia. 2023. Vol. 28. p. 101747.
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TY - JOUR
DO - 10.1016/j.mtla.2023.101747
UR - https://doi.org/10.1016/j.mtla.2023.101747
TI - Thermokinetic study of intermetallic phase formation in an Al/Cu multilayer thin film system
T2 - Materialia
AU - Moiseenko, Evgeny T
AU - Yumashev, V. V.
AU - Altunin, Roman R.
AU - Solovyov, Leonid A.
AU - Volochaev, Michail N
AU - Belousov, Oleg V.
AU - Zharkov, S. M.
PY - 2023
DA - 2023/05/01
PB - Elsevier
SP - 101747
VL - 28
SN - 2589-1529
ER -
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@article{2023_Moiseenko,
author = {Evgeny T Moiseenko and V. V. Yumashev and Roman R. Altunin and Leonid A. Solovyov and Michail N Volochaev and Oleg V. Belousov and S. M. Zharkov},
title = {Thermokinetic study of intermetallic phase formation in an Al/Cu multilayer thin film system},
journal = {Materialia},
year = {2023},
volume = {28},
publisher = {Elsevier},
month = {may},
url = {https://doi.org/10.1016/j.mtla.2023.101747},
pages = {101747},
doi = {10.1016/j.mtla.2023.101747}
}