Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6 (O)2 Piv10 } cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl
Elena Fursova
1, 2
,
Vladimir Ikorskii
1
,
Olga Kuznetsova
3
,
V. Ovcharenko
1
,
G. Romanenko
1
,
Igor L. Eremenko
4
,
Publication type: Journal Article
Publication date: 2007-06-01
scimago Q3
wos Q2
SJR: 0.396
CiteScore: 4.9
Impact factor: 2.6
ISSN: 02775387, 18733719
Materials Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The reaction of [Co6(O)2Piv10Thf3H2O] · 1.5Thf, where Piv=(CH3)3CCO2- and Thf = tetrahydrofuran, with nitroxides 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazole-3-oxide-1-oxyl (NIT-Me) and/or 2,4,4,5,5-pentamethyl-4,5-dihydro-1H -imidazole-1-oxyl (Im-Me) leads to simultaneous transformation of both the polymetallic core and the nitroxides. New polynuclear complexes: [Co9Piv12(OH)2L21]·0.5C7H16, [Co9Piv12(OH)2L21]·C7H16, [Co9Piv12(OH)2L21]·2C7H16, [Co8Piv8(OH)6(HPiv)4(H2O)2L24], L6[Co6(O)4Piv9(H2O)2] · 2HPiv, [Co6Piv8(HPiv)2L25], [Co6Piv8(HPiv)2L25]·C6H6,[Co6Piv8(HPiv)2L25][Co10Piv14(HPiv)2L22L23]·C7H16, and [Co10Piv14(HPiv)2L22L23]·C6H14 have been synthesized and characterized by X-ray crystallography; in these complexes, L1-L5 are modified molecules of the starting NIT-Me and/or Im-Me:
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Fursova E. et al. Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6(O)2Piv10} cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl // Polyhedron. 2007. Vol. 26. No. 9-11. pp. 2079-2088.
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Fursova E., Ikorskii V., Kuznetsova O., Ovcharenko V., Romanenko G., Eremenko I. L., Sidorov A. Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6(O)2Piv10} cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl // Polyhedron. 2007. Vol. 26. No. 9-11. pp. 2079-2088.
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TY - JOUR
DO - 10.1016/j.poly.2006.10.010
UR - https://doi.org/10.1016/j.poly.2006.10.010
TI - Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6(O)2Piv10} cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl
T2 - Polyhedron
AU - Fursova, Elena
AU - Ikorskii, Vladimir
AU - Kuznetsova, Olga
AU - Ovcharenko, V.
AU - Romanenko, G.
AU - Eremenko, Igor L.
AU - Sidorov, A.V
PY - 2007
DA - 2007/06/01
PB - Elsevier
SP - 2079-2088
IS - 9-11
VL - 26
SN - 0277-5387
SN - 1873-3719
ER -
Cite this
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@article{2007_Fursova,
author = {Elena Fursova and Vladimir Ikorskii and Olga Kuznetsova and V. Ovcharenko and G. Romanenko and Igor L. Eremenko and A.V Sidorov},
title = {Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6(O)2Piv10} cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl},
journal = {Polyhedron},
year = {2007},
volume = {26},
publisher = {Elsevier},
month = {jun},
url = {https://doi.org/10.1016/j.poly.2006.10.010},
number = {9-11},
pages = {2079--2088},
doi = {10.1016/j.poly.2006.10.010}
}
Cite this
MLA
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Fursova, Elena, et al. “Simultaneous transformation of a polynuclear complex and nitroxide in the reaction of the {Co6(O)2Piv10} cluster with 2,4,4,5,5-pentamethyl-4,5-dihydro-1H-imidazolyl-(3-oxide)-1-oxyl.” Polyhedron, vol. 26, no. 9-11, Jun. 2007, pp. 2079-2088. https://doi.org/10.1016/j.poly.2006.10.010.