Organic Letters, volume 22, issue 9, pages 3318-3322

Photoredox-Catalyzed Four-Component Reaction for the Synthesis of Complex Secondary Amines

Publication typeJournal Article
Publication date2020-03-11
Journal: Organic Letters
scimago Q1
wos Q1
SJR1.245
CiteScore9.3
Impact factor4.9
ISSN15237060, 15237052
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
The one-pot sulfonylation/aminoalkylation of styrene derivatives furnishing substituted γ-sulfonylamines was accomplished through a photoredox-catalyzed four-component reaction. Besides one molecule of water and the sodium counterion of the sulfinate, all atoms of the starting materials are transferred to the final product, rendering this process highly atom-efficient. The operationally simple protocol allows for the simultaneous formation of three new single bonds (C-S, C-N, and C-C) and therefore grants rapid access to structurally diverse products.
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