Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters
Publication type: Journal Article
Publication date: 2001-02-02
scimago Q1
wos Q1
SJR: 1.533
CiteScore: 11.6
Impact factor: 6.7
ISSN: 00032700, 15206882, 21542686
PubMed ID:
11289437
Analytical Chemistry
Abstract
Monolayer-protected Au clusters (MPCs) have been prepared with mixed monolayers of alkanethiolates and alkanethiolates terminally omega-functionalized with phenothiazine. The mixed monolayer MPCs can contain as many as 10 phenothiazines/MPC; these electron donors are electroactive in rapid, successive one-electron reactions. Surface adsorption of the functionalized MPCs is evident in cyclic voltammetry. Double-potential-step chronocoulometry with incremented potential steps was applied to unfunctionalized hexanethiolate-coated MPCs and to those functionalized with phenothiazine to analyze the coupling between the diffusion-controlled double-layer charging of the MPC cores and the oxidation of the phenothiazine centers. Apparent changes in ordering of the MPC alkanethiolate chains were observed with infrared spectroscopy in solutions of MPCs where alcohol, carboxylic acid, or phenothiazine moieties had been incorporated into the monolayer.
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Total citations:
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Citations from 2024:
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Miles D. T., Murray R. W. Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters // Analytical Chemistry. 2001. Vol. 73. No. 5. pp. 921-929.
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Miles D. T., Murray R. W. Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters // Analytical Chemistry. 2001. Vol. 73. No. 5. pp. 921-929.
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RIS
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TY - JOUR
DO - 10.1021/ac0012647
UR - https://doi.org/10.1021/ac0012647
TI - Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters
T2 - Analytical Chemistry
AU - Miles, Deon T.
AU - Murray, Royce W.
PY - 2001
DA - 2001/02/02
PB - American Chemical Society (ACS)
SP - 921-929
IS - 5
VL - 73
PMID - 11289437
SN - 0003-2700
SN - 1520-6882
SN - 2154-2686
ER -
Cite this
BibTex (up to 50 authors)
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@article{2001_Miles,
author = {Deon T. Miles and Royce W. Murray},
title = {Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters},
journal = {Analytical Chemistry},
year = {2001},
volume = {73},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/ac0012647},
number = {5},
pages = {921--929},
doi = {10.1021/ac0012647}
}
Cite this
MLA
Copy
Miles, Deon T., and Royce W. Murray. “Redox and Double-Layer Charging of Phenothiazine Functionalized Monolayer-Protected Clusters.” Analytical Chemistry, vol. 73, no. 5, Feb. 2001, pp. 921-929. https://doi.org/10.1021/ac0012647.