Journal of Physical Chemistry C, volume 125, issue 8, pages 4694-4703
Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study
Publication type: Journal Article
Publication date: 2021-02-22
Journal:
Journal of Physical Chemistry C
Quartile SCImago
Q1
Quartile WOS
Q2
Impact factor: 3.7
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
Conventional infrared spectroscopy is widely used to analyze the structural properties of compounds in the fingerprint region. However, a precise spectroscopic study of thin films is a nontrivial task due to the small absorption cross sections of analytes. In this regard, surface-enhanced infrared absorption (SEIRA) spectroscopy can be applied to overcome the limitation by the near-field enhancement of plasmonic metasurfaces. Here we present for the first time the SEIRA study of the widely used organic optoelectronic material Tris(8-hydroxyquinoline) aluminum(III) (Alq3). A special design of the metasurfaces based on arrays of gold Y-shaped nanoantennas is developed for the SEIRA study of Alq3 thermally deposited layers with film thickness growth. This design supports two independent plasmonic resonances for each metasurface and makes it possible to use one SEIRA substrate for the precise study of several vibrational modes of the compound. Observed near-field enhancement of the fabricated metasurfaces revealed a saturation and a diminishing in signal with the analyte layer thickness from half the height of gold nanoantennas onward. This effect is associated with Alq3 side accumulation as shown by atomic force microscopy. A fabricated SEIRA substrate indicates the possibilities for further progress of spectroscopic chemical imaging in optoelectronics and is especially promising for organic electronic devices that consist of multiple layers of transport materials.
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Physical Chemistry Chemical Physics
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Citations by publishers
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1
2
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Springer Nature
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Springer Nature
2 publications, 25%
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IOP Publishing
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IOP Publishing
2 publications, 25%
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Wiley
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Wiley
1 publication, 12.5%
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Walter de Gruyter
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Walter de Gruyter
1 publication, 12.5%
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IEEE
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IEEE
1 publication, 12.5%
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Royal Society of Chemistry (RSC)
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Royal Society of Chemistry (RSC)
1 publication, 12.5%
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1
2
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- Statistics recalculated weekly.
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Zvagelsky R. et al. Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study // Journal of Physical Chemistry C. 2021. Vol. 125. No. 8. pp. 4694-4703.
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Zvagelsky R., Chubich D., Pisarenko A., Bedran Z., Zhukova E. S. Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study // Journal of Physical Chemistry C. 2021. Vol. 125. No. 8. pp. 4694-4703.
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TY - JOUR
DO - 10.1021/acs.jpcc.0c10433
UR - https://doi.org/10.1021%2Facs.jpcc.0c10433
TI - Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study
T2 - Journal of Physical Chemistry C
AU - Chubich, Dmytro
AU - Pisarenko, Anastasia
AU - Bedran, Zakhar
AU - Zvagelsky, R.D.
AU - Zhukova, Elena S.
PY - 2021
DA - 2021/02/22 00:00:00
PB - American Chemical Society (ACS)
SP - 4694-4703
IS - 8
VL - 125
SN - 1932-7447
SN - 1932-7455
ER -
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@article{2021_Zvagelsky,
author = {Dmytro Chubich and Anastasia Pisarenko and Zakhar Bedran and R.D. Zvagelsky and Elena S. Zhukova},
title = {Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study},
journal = {Journal of Physical Chemistry C},
year = {2021},
volume = {125},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021%2Facs.jpcc.0c10433},
number = {8},
pages = {4694--4703},
doi = {10.1021/acs.jpcc.0c10433}
}
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MLA
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Zvagelsky, R.D., et al. “Plasmonic Metasurfaces as Surface-Enhanced Infrared Absorption Substrates for Optoelectronics: Alq3 Thin-Film Study.” Journal of Physical Chemistry C, vol. 125, no. 8, Feb. 2021, pp. 4694-4703. https://doi.org/10.1021%2Facs.jpcc.0c10433.