Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts
Publication type: Journal Article
Publication date: 2018-06-20
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
The elucidation of structure–property relationships for supported metal catalysts requires atomic-scale descriptions and quantitative measurements of the relative population of various exposed active sites under reaction conditions. The requirement of describing catalyst structures under reaction conditions stems from the potential physical and chemical reconstruction that can be induced by changes in environment. Here we highlight our recent work, where catalyst characterization via a combination of in-situ transmission electron microscopy and infrared spectroscopy is used to provide sample-averaged, site-specific atomic level information on supported metal catalysts under reaction conditions. We show two illustrative examples using different reaction systems: the oxidation of CO over supported Pt and the reduction of CO2 over supported Rh. Using these examples we demonstrate differentiation of the catalytic reactivity of small supported metal clusters from isolated atoms and interrogate the catalytic co...
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Total citations:
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Citations from 2024:
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(26%)
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GOST
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Resasco J. et al. Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts // Journal of Physical Chemistry C. 2018. Vol. 122. No. 44. pp. 25143-25157.
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Resasco J., Dai S., GRAHAM G., Pan X., Christopher P. Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts // Journal of Physical Chemistry C. 2018. Vol. 122. No. 44. pp. 25143-25157.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.jpcc.8b03959
UR - https://doi.org/10.1021/acs.jpcc.8b03959
TI - Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts
T2 - Journal of Physical Chemistry C
AU - Resasco, Joaquin
AU - Dai, Sheng
AU - GRAHAM, GEORGE
AU - Pan, Xiaoqing
AU - Christopher, Phillip
PY - 2018
DA - 2018/06/20
PB - American Chemical Society (ACS)
SP - 25143-25157
IS - 44
VL - 122
SN - 1932-7447
SN - 1932-7455
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2018_Resasco,
author = {Joaquin Resasco and Sheng Dai and GEORGE GRAHAM and Xiaoqing Pan and Phillip Christopher},
title = {Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts},
journal = {Journal of Physical Chemistry C},
year = {2018},
volume = {122},
publisher = {American Chemical Society (ACS)},
month = {jun},
url = {https://doi.org/10.1021/acs.jpcc.8b03959},
number = {44},
pages = {25143--25157},
doi = {10.1021/acs.jpcc.8b03959}
}
Cite this
MLA
Copy
Resasco, Joaquin, et al. “Combining In-Situ Transmission Electron Microscopy and Infrared Spectroscopy for Understanding Dynamic and Atomic-Scale Features of Supported Metal Catalysts.” Journal of Physical Chemistry C, vol. 122, no. 44, Jun. 2018, pp. 25143-25157. https://doi.org/10.1021/acs.jpcc.8b03959.