Langmuir, volume 38, issue 33, pages 10202-10215
Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases
Publication type: Journal Article
Publication date: 2022-08-11
PubMed ID:
35951972
Spectroscopy
Electrochemistry
Condensed Matter Physics
General Materials Science
Surfaces and Interfaces
Abstract
We have studied decanethiolate self-assembled monolayers on the Au(001) surface. Planar and striped phases, as well as disordered regions, have formed after exposing the Au surface to a decanethiol solution. The planar phases that we observe have a hexagonal symmetry and have not been previously reported for thiols on the Au(001) surface and have lower coverage compared to that of the other known thiol planar phases such as the square α phase. The striped phases that we observe are similar to the previously reported β phase but still feature unit cells that cannot be modeled as the archetype, and the coverage is also somewhat lower. The disordered decanethiolate regions are more dynamic compared to the ordered phases, confirmed with I(t) spectroscopy. This suggests that in these regions the coverage is too low in order to form ordered decanethiolate phases. Our findings contribute to the growing family of possible decanethiol formations on the Au(001) surface, for which still less is known compared to the extensive overview present for the Au(111) surface.
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Tsvetanova M. et al. Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases // Langmuir. 2022. Vol. 38. No. 33. pp. 10202-10215.
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Tsvetanova M., Syromyatnikov A. G., Van Der Meer T., van Houselt A., Houselt A. V., Klavsyuk A. L., Sotthewes K. Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases // Langmuir. 2022. Vol. 38. No. 33. pp. 10202-10215.
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TY - JOUR
DO - 10.1021/acs.langmuir.2c01356
UR - https://doi.org/10.1021/acs.langmuir.2c01356
TI - Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases
T2 - Langmuir
AU - Van Der Meer, Thomas
AU - Klavsyuk, Andrey L.
AU - Tsvetanova, Martina
AU - Syromyatnikov, Alexey G.
AU - van Houselt, Arie
AU - Houselt, Arie Van
AU - Sotthewes, K.
PY - 2022
DA - 2022/08/11
PB - American Chemical Society (ACS)
SP - 10202-10215
IS - 33
VL - 38
PMID - 35951972
SN - 0743-7463
SN - 1520-5827
ER -
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@article{2022_Tsvetanova,
author = {Thomas Van Der Meer and Andrey L. Klavsyuk and Martina Tsvetanova and Alexey G. Syromyatnikov and Arie van Houselt and Arie Van Houselt and K. Sotthewes},
title = {Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases},
journal = {Langmuir},
year = {2022},
volume = {38},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.langmuir.2c01356},
number = {33},
pages = {10202--10215},
doi = {10.1021/acs.langmuir.2c01356}
}
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Tsvetanova, Martina, et al. “Self-Assembled Decanethiolate Monolayers on Au(001): Expanding the Family of Known Phases.” Langmuir, vol. 38, no. 33, Aug. 2022, pp. 10202-10215. https://doi.org/10.1021/acs.langmuir.2c01356.