volume 24 issue 1 pages 152-157

Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes

Publication typeJournal Article
Publication date2021-12-21
scimago Q1
wos Q1
SJR1.235
CiteScore8.7
Impact factor5.0
ISSN15237060, 15237052
Organic Chemistry
Biochemistry
Physical and Theoretical Chemistry
Abstract
A general synthetic entry to functionalized dihydrophenalenes has been found using naphthyl-cyclopropane esters as starting materials. The desired annulation was possible with visible light, Ir(Fppy)3 as photocatalyst, BnNMe2 or DABCO as electron donor, HAT-catalyst, and proton source. A broad scope of substituted naphthyl and azanaphthyl derivatives provided the photoannulation products in high yield. Deuteration studies support a photoredox mechanism involving the photoreductive cyclopropane opening to an enolate radical followed by an aryl radical trapping.
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Schmalz V., Koert U. Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes // Organic Letters. 2021. Vol. 24. No. 1. pp. 152-157.
GOST all authors (up to 50) Copy
Schmalz V., Koert U. Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes // Organic Letters. 2021. Vol. 24. No. 1. pp. 152-157.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.orglett.1c03784
UR - https://doi.org/10.1021/acs.orglett.1c03784
TI - Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes
T2 - Organic Letters
AU - Schmalz, Veronika
AU - Koert, Ulrich
PY - 2021
DA - 2021/12/21
PB - American Chemical Society (ACS)
SP - 152-157
IS - 1
VL - 24
PMID - 34932368
SN - 1523-7060
SN - 1523-7052
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2021_Schmalz,
author = {Veronika Schmalz and Ulrich Koert},
title = {Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes},
journal = {Organic Letters},
year = {2021},
volume = {24},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.orglett.1c03784},
number = {1},
pages = {152--157},
doi = {10.1021/acs.orglett.1c03784}
}
MLA
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MLA Copy
Schmalz, Veronika, and Ulrich Koert. “Visible-Light-Induced Photoannulation of α-Naphthyl Cyclopropane Carboxylic Esters to Functionalized Dihydrophenalenes.” Organic Letters, vol. 24, no. 1, Dec. 2021, pp. 152-157. https://doi.org/10.1021/acs.orglett.1c03784.