Journal of the American Chemical Society, volume 131, issue 1, pages 50-51

Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments

Yuanjian Zhang ¹

Arne Thomas ¹

Markus Antonietti ¹

Xinchen Wang ¹

Hide authors affiliations Show authors affiliations: 1 affiliation

Max Planck Institute of Colloids and Interfaces, Research Campus Golm, D-14424 Potsdam, Germany |

Publication type: Journal Article

Publication date: 2008-12-10

American Chemical Society (ACS)

Journal: Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

Impact factor: 15

ISSN: 00027863, 15205126

DOI: 10.1021/ja808329f

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General Chemistry

Catalysis

Biochemistry

Colloid and Surface Chemistry

Abstract

Covalently bonded carbon nitride materials (e.g., g-C(3)N(4)) have numerous potential applications ranging from semiconductors to fuel cells. But their solubility is poor, which makes characterization and processing difficult. Moreover, the chemistry of the as-synthesized carbon nitrides has been widely neglected. Here we report that some of these handicaps might be overcome by a controllable and reversible protonation. It was found that protonation not only provides better dispersion and exposes a high surface area for g-C(3)N(4) but also enables an adjustment of electronic band gaps and higher ionic conductivity. Recovery or deprotonation toward the original g-C(3)N(4) could be obtained by simple heating, which enables improved sintering but also a potential preservation of the higher surface area of the protonated material. This proton-enhanced sintering process allowed for the first time direct measurement of the photoconductivity of the material. By aid of protonation, other promising g-C(3)N(4) based hybrid composites could also be facilely obtained by simple counteranion exchange.

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Citations by journals

	5 10 15 20 25 30
Applied Surface Science	Applied Surface Science, 29, 4.08% Applied Surface Science 29 publications, 4.08%
RSC Advances	RSC Advances, 29, 4.08% RSC Advances 29 publications, 4.08%
Applied Catalysis B: Environmental	Applied Catalysis B: Environmental, 27, 3.8% Applied Catalysis B: Environmental 27 publications, 3.8%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 26, 3.66% Journal of Materials Chemistry A 26 publications, 3.66%
ACS applied materials & interfaces	ACS applied materials & interfaces, 17, 2.39% ACS applied materials & interfaces 17 publications, 2.39%
Physical Chemistry Chemical Physics	Physical Chemistry Chemical Physics, 17, 2.39% Physical Chemistry Chemical Physics 17 publications, 2.39%
International Journal of Hydrogen Energy	International Journal of Hydrogen Energy, 15, 2.11% International Journal of Hydrogen Energy 15 publications, 2.11%
Angewandte Chemie - International Edition	Angewandte Chemie - International Edition, 15, 2.11% Angewandte Chemie - International Edition 15 publications, 2.11%
Angewandte Chemie	Angewandte Chemie, 15, 2.11% Angewandte Chemie 15 publications, 2.11%
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 13, 1.83% Journal of Alloys and Compounds 13 publications, 1.83%
Chemical Engineering Journal	Chemical Engineering Journal, 11, 1.55% Chemical Engineering Journal 11 publications, 1.55%
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Electrochimica Acta	Electrochimica Acta, 10, 1.41% Electrochimica Acta 10 publications, 1.41%
ChemSusChem	ChemSusChem, 10, 1.41% ChemSusChem 10 publications, 1.41%
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Chemical Communications	Chemical Communications, 10, 1.41% Chemical Communications 10 publications, 1.41%
New Journal of Chemistry	New Journal of Chemistry, 10, 1.41% New Journal of Chemistry 10 publications, 1.41%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 9, 1.27% Journal of Physical Chemistry C 9 publications, 1.27%
Advanced Functional Materials	Advanced Functional Materials, 9, 1.27% Advanced Functional Materials 9 publications, 1.27%
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Small	Small, 8, 1.13% Small 8 publications, 1.13%
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Materials Research Bulletin	Materials Research Bulletin, 7, 0.99% Materials Research Bulletin 7 publications, 0.99%
Advanced Materials	Advanced Materials, 7, 0.99% Advanced Materials 7 publications, 0.99%
ChemCatChem	ChemCatChem, 7, 0.99% ChemCatChem 7 publications, 0.99%
Nanoscale	Nanoscale, 7, 0.99% Nanoscale 7 publications, 0.99%
Journal of the American Chemical Society	Journal of the American Chemical Society, 6, 0.85% Journal of the American Chemical Society 6 publications, 0.85%
Nature Communications	Nature Communications, 6, 0.85% Nature Communications 6 publications, 0.85%
	5 10 15 20 25 30

Citations by publishers

	50 100 150 200 250 300
Elsevier	Elsevier, 276, 38.87% Elsevier 276 publications, 38.87%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 143, 20.14% Royal Society of Chemistry (RSC) 143 publications, 20.14%
Wiley	Wiley, 122, 17.18% Wiley 122 publications, 17.18%
American Chemical Society (ACS)	American Chemical Society (ACS), 79, 11.13% American Chemical Society (ACS) 79 publications, 11.13%
Springer Nature	Springer Nature, 30, 4.23% Springer Nature 30 publications, 4.23%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 12, 1.69% Multidisciplinary Digital Publishing Institute (MDPI) 12 publications, 1.69%
The Electrochemical Society	The Electrochemical Society, 4, 0.56% The Electrochemical Society 4 publications, 0.56%
IOP Publishing	IOP Publishing, 4, 0.56% IOP Publishing 4 publications, 0.56%
Trans Tech Publications	Trans Tech Publications, 4, 0.56% Trans Tech Publications 4 publications, 0.56%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 3, 0.42% American Institute of Physics (AIP) 3 publications, 0.42%
Frontiers Media S.A.	Frontiers Media S.A., 3, 0.42% Frontiers Media S.A. 3 publications, 0.42%
Korean Society of Industrial Engineering Chemistry	Korean Society of Industrial Engineering Chemistry, 3, 0.42% Korean Society of Industrial Engineering Chemistry 3 publications, 0.42%
Taylor & Francis	Taylor & Francis, 3, 0.42% Taylor & Francis 3 publications, 0.42%
Electrochemical Science Group, University of Belgrade	Electrochemical Science Group, University of Belgrade, 3, 0.42% Electrochemical Science Group, University of Belgrade 3 publications, 0.42%
SAGE	SAGE, 2, 0.28% SAGE 2 publications, 0.28%
Japan Society of Applied Physics	Japan Society of Applied Physics, 2, 0.28% Japan Society of Applied Physics 2 publications, 0.28%
IOS Press	IOS Press, 2, 0.28% IOS Press 2 publications, 0.28%
Beilstein-Institut	Beilstein-Institut, 1, 0.14% Beilstein-Institut 1 publication, 0.14%
American Physical Society (APS)	American Physical Society (APS), 1, 0.14% American Physical Society (APS) 1 publication, 0.14%
The Chemical Society of Japan	The Chemical Society of Japan, 1, 0.14% The Chemical Society of Japan 1 publication, 0.14%
Institution of Engineering and Technology (IET)	Institution of Engineering and Technology (IET), 1, 0.14% Institution of Engineering and Technology (IET) 1 publication, 0.14%
IWA Publishing	IWA Publishing, 1, 0.14% IWA Publishing 1 publication, 0.14%
Nonferrous Metals Society of China	Nonferrous Metals Society of China, 1, 0.14% Nonferrous Metals Society of China 1 publication, 0.14%
Taiwan Institute of Chemical Engineers	Taiwan Institute of Chemical Engineers, 1, 0.14% Taiwan Institute of Chemical Engineers 1 publication, 0.14%
Chinese Society of Rare Earths	Chinese Society of Rare Earths, 1, 0.14% Chinese Society of Rare Earths 1 publication, 0.14%
Pleiades Publishing	Pleiades Publishing, 1, 0.14% Pleiades Publishing 1 publication, 0.14%
Walter de Gruyter	Walter de Gruyter, 1, 0.14% Walter de Gruyter 1 publication, 0.14%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.14% American Association for the Advancement of Science (AAAS) 1 publication, 0.14%
Hans Publishers	Hans Publishers, 1, 0.14% Hans Publishers 1 publication, 0.14%
	50 100 150 200 250 300

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Zhang Y. et al. Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments // Journal of the American Chemical Society. 2008. Vol. 131. No. 1. pp. 50-51.

GOST all authors (up to 50) Copy

Zhang Y., Thomas A., Antonietti M., Wang X. Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments // Journal of the American Chemical Society. 2008. Vol. 131. No. 1. pp. 50-51.

RIS |

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RIS Copy

TY - JOUR

DO - 10.1021/ja808329f

UR - https://doi.org/10.1021/ja808329f

TI - Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments

T2 - Journal of the American Chemical Society

AU - Zhang, Yuanjian

AU - Thomas, Arne

AU - Antonietti, Markus

AU - Wang, Xinchen

PY - 2008

DA - 2008/12/10 00:00:00

PB - American Chemical Society (ACS)

SP - 50-51

IS - 1

VL - 131

SN - 0002-7863

SN - 1520-5126

ER -

BibTex |

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BibTex Copy

@article{2008_Zhang,

author = {Yuanjian Zhang and Arne Thomas and Markus Antonietti and Xinchen Wang},

title = {Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments},

journal = {Journal of the American Chemical Society},

year = {2008},

volume = {131},

publisher = {American Chemical Society (ACS)},

month = {dec},

url = {https://doi.org/10.1021/ja808329f},

number = {1},

pages = {50--51},

doi = {10.1021/ja808329f}

}

MLA

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MLA Copy

Zhang, Yuanjian, et al. “Activation of Carbon Nitride Solids by Protonation: Morphology Changes, Enhanced Ionic Conductivity, and Photoconduction Experiments.” Journal of the American Chemical Society, vol. 131, no. 1, Dec. 2008, pp. 50-51. https://doi.org/10.1021/ja808329f.

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Publisher

American Chemical Society (ACS)

Journal

Journal of the American Chemical Society

Quartile SCImago

Quartile WOS

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ISSN

00027863 (Print)
15205126 (Electronic)