A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis
Publication type: Journal Article
Publication date: 2023-11-07
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
37934955
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Covalent organic frameworks (COFs) have emerged as tunable, crystalline, and porous functional organic materials, but their application in photocatalysis has been limited by rapid excited-state quenching. Herein, we report the first example of dual photoredox/nickel catalysis by an sp2 carbon-conjugated spirobifluorene-based COF. Constructed from spirobifluorene and nickel-bipyridine linkers, the NiSCN COF adopted a two-dimensional structure with staggered stacking. Under light irradiation, NiSCN catalyzed amination and etherification/esterification reactions of aryl halides through the photoredox mechanism, with a catalytic efficiency more than 23-fold higher than that of its homogeneous control. NiSCN was used in five consecutive reactions without a significant loss of catalytic activity.
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64
Total citations:
64
Citations from 2024:
63
(98.44%)
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GOST
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Fan Y. et al. A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis // Journal of the American Chemical Society. 2023. Vol. 145. No. 46. pp. 25074-25079.
GOST all authors (up to 50)
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Fan Y., Kang D. W., Labalme S., Lin W. A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis // Journal of the American Chemical Society. 2023. Vol. 145. No. 46. pp. 25074-25079.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.3c09729
UR - https://pubs.acs.org/doi/10.1021/jacs.3c09729
TI - A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis
T2 - Journal of the American Chemical Society
AU - Fan, Yingjie
AU - Kang, Dong Won
AU - Labalme, Steven
AU - Lin, Wenbin
PY - 2023
DA - 2023/11/07
PB - American Chemical Society (ACS)
SP - 25074-25079
IS - 46
VL - 145
PMID - 37934955
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2023_Fan,
author = {Yingjie Fan and Dong Won Kang and Steven Labalme and Wenbin Lin},
title = {A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis},
journal = {Journal of the American Chemical Society},
year = {2023},
volume = {145},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://pubs.acs.org/doi/10.1021/jacs.3c09729},
number = {46},
pages = {25074--25079},
doi = {10.1021/jacs.3c09729}
}
Cite this
MLA
Copy
Fan, Yingjie, et al. “A Spirobifluorene-Based Covalent Organic Framework for Dual Photoredox and Nickel Catalysis.” Journal of the American Chemical Society, vol. 145, no. 46, Nov. 2023, pp. 25074-25079. https://pubs.acs.org/doi/10.1021/jacs.3c09729.
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