Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B
Publication type: Journal Article
Publication date: 2019-11-26
scimago Q1
wos Q1
SJR: 5.554
CiteScore: 22.5
Impact factor: 15.6
ISSN: 00027863, 15205126
PubMed ID:
31770485
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
We present a bioinspired late-stage C–H oxidation of the ent-trachylobane natural product mitrephorone B to mitrephorone A. The realization of this unprecedented transformation was accomplished by either an iron-catalyzed or electrochemical oxidation and enabled access to the densely substituted oxetane in one step. Formation of mitrephorone C, which is lacking the central oxetane unit but features a keto-function at C2, was not formed under these conditions.
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Total citations:
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Citations from 2024:
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(26.09%)
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GOST
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Wein L. A. et al. Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B // Journal of the American Chemical Society. 2019. Vol. 141. No. 50. pp. 19589-19593.
GOST all authors (up to 50)
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Wein L. A., Wurst K., Angyal P., Weisheit L., Magauer T. Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B // Journal of the American Chemical Society. 2019. Vol. 141. No. 50. pp. 19589-19593.
Cite this
RIS
Copy
TY - JOUR
DO - 10.1021/jacs.9b11646
UR - https://doi.org/10.1021/jacs.9b11646
TI - Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B
T2 - Journal of the American Chemical Society
AU - Wein, Lukas Anton
AU - Wurst, Klaus
AU - Angyal, Péter
AU - Weisheit, Lara
AU - Magauer, Thomas
PY - 2019
DA - 2019/11/26
PB - American Chemical Society (ACS)
SP - 19589-19593
IS - 50
VL - 141
PMID - 31770485
SN - 0002-7863
SN - 1520-5126
ER -
Cite this
BibTex (up to 50 authors)
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@article{2019_Wein,
author = {Lukas Anton Wein and Klaus Wurst and Péter Angyal and Lara Weisheit and Thomas Magauer},
title = {Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B},
journal = {Journal of the American Chemical Society},
year = {2019},
volume = {141},
publisher = {American Chemical Society (ACS)},
month = {nov},
url = {https://doi.org/10.1021/jacs.9b11646},
number = {50},
pages = {19589--19593},
doi = {10.1021/jacs.9b11646}
}
Cite this
MLA
Copy
Wein, Lukas Anton, et al. “Synthesis of (−)-Mitrephorone A via a Bioinspired Late Stage C–H Oxidation of (−)-Mitrephorone B.” Journal of the American Chemical Society, vol. 141, no. 50, Nov. 2019, pp. 19589-19593. https://doi.org/10.1021/jacs.9b11646.