Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes
Publication type: Journal Article
Publication date: 2013-07-16
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
23859100
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The selective syntheses of new classes of 6,9-dialkenyl- and 6-alkenyl-decaboranes and 6-alkyl-9-alkenyl-decaboranes have been achieved via iridium and ruthenium catalyzed decaborane and 6-alkyl-decaborane alkyne-hydroborations. Reactions employing [Cp*IrCl2]2 and [RuCl2(p-cymene)]2 precatalysts gave β-E-alkenyl-decaboranes, while the corresponding reactions with [RuI2(p-cymene)]2 gave the α-alkenyl-decaborane isomers, with the differences in product selectivity suggesting quite different mechanistic steps for the catalysts. The alkenyl-decaboranes were easily converted to other useful derivatives, including coupled-cage and functionally substituted compounds, via iridium-catalyzed hydroborations and ruthenium-catalyzed homo and cross olefin-metathesis reactions.
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Chatterjee S., Carroll P., Sneddon L. G. Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes // Inorganic Chemistry. 2013. Vol. 52. No. 15. pp. 9119-9130.
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Chatterjee S., Carroll P., Sneddon L. G. Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes // Inorganic Chemistry. 2013. Vol. 52. No. 15. pp. 9119-9130.
Cite this
RIS
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TY - JOUR
DO - 10.1021/ic401356u
UR - https://doi.org/10.1021/ic401356u
TI - Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes
T2 - Inorganic Chemistry
AU - Chatterjee, Shahana
AU - Carroll, Patrick
AU - Sneddon, Larry G.
PY - 2013
DA - 2013/07/16
PB - American Chemical Society (ACS)
SP - 9119-9130
IS - 15
VL - 52
PMID - 23859100
SN - 0020-1669
SN - 1520-510X
ER -
Cite this
BibTex (up to 50 authors)
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@article{2013_Chatterjee,
author = {Shahana Chatterjee and Patrick Carroll and Larry G. Sneddon},
title = {Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes},
journal = {Inorganic Chemistry},
year = {2013},
volume = {52},
publisher = {American Chemical Society (ACS)},
month = {jul},
url = {https://doi.org/10.1021/ic401356u},
number = {15},
pages = {9119--9130},
doi = {10.1021/ic401356u}
}
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MLA
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Chatterjee, Shahana, et al. “Iridium and Ruthenium Catalyzed Syntheses, Hydroborations, and Metathesis Reactions of Alkenyl-Decaboranes.” Inorganic Chemistry, vol. 52, no. 15, Jul. 2013, pp. 9119-9130. https://doi.org/10.1021/ic401356u.