Journal of the American Chemical Society, volume 133, issue 11, pages 3964-3971
Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania.
Nada M. Dimitrijevic
1
,
Baiju Vijayan
2
,
Oleg G. Poluektov
3
,
Tijana Rajh
3
,
Kimberly Gray
2
,
Haiying He
3
,
Publication type: Journal Article
Publication date: 2011-02-24
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 15
ISSN: 00027863, 15205126
General Chemistry
Catalysis
Biochemistry
Colloid and Surface Chemistry
Abstract
Using the electron paramagnetic resonance technique, we have elucidated the multiple roles of water and carbonates in the overall photocatalytic reduction of carbon dioxide to methane over titania nanoparticles. The formation of H atoms (reduction product) and (•)OH radicals (oxidation product) from water, and CO(3)(-) radical anions (oxidation product) from carbonates, was detected in CO(2)-saturated titania aqueous dispersion under UV illumination. Additionally, methoxyl, (•)OCH(3), and methyl, (•)CH(3), radicals were identified as reaction intermediates. The two-electron, one-proton reaction proposed as an initial step in the reduction of CO(2) on the surface of TiO(2) is supported by the results of first-principles calculations.
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1 publication, 0.24%
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20
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160
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Dimitrijevic N. M. et al. Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania. // Journal of the American Chemical Society. 2011. Vol. 133. No. 11. pp. 3964-3971.
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Dimitrijevic N. M., Vijayan B., Poluektov O. G., Rajh T., Gray K., He H., Zapol P. Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania. // Journal of the American Chemical Society. 2011. Vol. 133. No. 11. pp. 3964-3971.
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TY - JOUR
DO - 10.1021/ja108791u
UR - https://doi.org/10.1021/ja108791u
TI - Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania.
T2 - Journal of the American Chemical Society
AU - Dimitrijevic, Nada M.
AU - Poluektov, Oleg G.
AU - Vijayan, Baiju
AU - Rajh, Tijana
AU - Gray, Kimberly
AU - He, Haiying
AU - Zapol, Peter
PY - 2011
DA - 2011/02/24 00:00:00
PB - American Chemical Society (ACS)
SP - 3964-3971
IS - 11
VL - 133
SN - 0002-7863
SN - 1520-5126
ER -
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@article{2011_Dimitrijevic,
author = {Nada M. Dimitrijevic and Oleg G. Poluektov and Baiju Vijayan and Tijana Rajh and Kimberly Gray and Haiying He and Peter Zapol},
title = {Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania.},
journal = {Journal of the American Chemical Society},
year = {2011},
volume = {133},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/ja108791u},
number = {11},
pages = {3964--3971},
doi = {10.1021/ja108791u}
}
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Dimitrijevic, Nada M., et al. “Role of water and carbonates in photocatalytic transformation of CO2 to CH4 on titania..” Journal of the American Chemical Society, vol. 133, no. 11, Feb. 2011, pp. 3964-3971. https://doi.org/10.1021/ja108791u.