Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands
Тип публикации: Journal Article
Дата публикации: 2008-02-19
SCImago Q2
WOS Q2
БС1
SJR: 0.55
CiteScore: 4.6
Impact factor: 2.4
ISSN: 02767333, 15206041
Organic Chemistry
Inorganic Chemistry
Physical and Theoretical Chemistry
Краткое описание
A total of nine Walphos-type diphosphine ligands, all of which have a ferrocenyl-aryl backbone, have been synthesized, characterized, and tested in asymmetric ruthenium-, rhodium-, and iridium-catalyzed hydrogenations of alkenes, ketones, and one imine. Ruthenium- and rhodium-mediated hydrogenations of alkenes and ketones gave enantioselectivities of up to 95% and 97% ee, respectively. Ligand tuning was attempted by variation of the phosphorus-bound aryl and alkyl substituents and by attaching electron-donating or electron-withdrawing substituents to the backbone phenyl ring. Dichloropalladium(II) complexes of five ligands were synthesized, and in four cases the molecular structures were studied in solution as well as in the solid state.
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ГОСТ
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Wang Y. et al. Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands // Organometallics. 2008. Vol. 27. No. 6. pp. 1119-1127.
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Wang Y., Sturm T., Steurer M., Arion V. B., Mereiter K., Spindler F., Weissensteiner W. Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands // Organometallics. 2008. Vol. 27. No. 6. pp. 1119-1127.
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TY - JOUR
DO - 10.1021/om701103d
UR - https://doi.org/10.1021/om701103d
TI - Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands
T2 - Organometallics
AU - Wang, Yaping
AU - Sturm, Thomas
AU - Steurer, Marianne
AU - Arion, Vladimir B.
AU - Mereiter, K.
AU - Spindler, Felix
AU - Weissensteiner, Walter
PY - 2008
DA - 2008/02/19
PB - American Chemical Society (ACS)
SP - 1119-1127
IS - 6
VL - 27
SN - 0276-7333
SN - 1520-6041
ER -
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BibTex (до 50 авторов)
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@article{2008_Wang,
author = {Yaping Wang and Thomas Sturm and Marianne Steurer and Vladimir B. Arion and K. Mereiter and Felix Spindler and Walter Weissensteiner},
title = {Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands},
journal = {Organometallics},
year = {2008},
volume = {27},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/om701103d},
number = {6},
pages = {1119--1127},
doi = {10.1021/om701103d}
}
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MLA
Скопировать
Wang, Yaping, et al. “Synthesis, Coordination Behavior, and Use in Asymmetric Hydrogenations of Walphos-Type Ligands.” Organometallics, vol. 27, no. 6, Feb. 2008, pp. 1119-1127. https://doi.org/10.1021/om701103d.
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