volume 17 issue 3 pages 1353-1362

H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes

Publication typeJournal Article
Publication date2017-02-01
scimago Q2
wos Q1
SJR0.633
CiteScore5.6
Impact factor3.4
ISSN15287483, 15287505
General Chemistry
Condensed Matter Physics
General Materials Science
Abstract
The dihalomethane–halide H2C(X)–X···X– (X = Cl, Br) halogen bonding was detected in a series of the cis-[PdX(CNCy){C(NHCy)═NHC6H2Me2NH2}]X•CH2X2 (X = Cl, Br) associates by single-crystal XRD followed by DFT calculations. Although ESP calculations demonstrated that the σ-hole of dichloromethane is the smallest among all halomethane solvents (the maximum electrostatic potential is only 2.6 kcal/mol), the theoretical DFT calculations followed by Bader’s QTAIM analysis (M06/DZP-DKH level of theory) confirmed the H2C(X)–X···X– halogen bond in both the solid-state and gas-phase optimized geometries. The estimated bonding energy in H2C(X)–X···X– is in the 1.9–2.8 kcal/mol range.
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Ivanov D. M. et al. H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes // Crystal Growth and Design. 2017. Vol. 17. No. 3. pp. 1353-1362.
GOST all authors (up to 50) Copy
Ivanov D. M., Kinzhalov M. A., Novikov A. S., Ananyev I. V., Romanova A. A., Boyarskiy V. P., Haukka M., Kukushkin V. Y. H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes // Crystal Growth and Design. 2017. Vol. 17. No. 3. pp. 1353-1362.
RIS |
Cite this
RIS Copy
TY - JOUR
DO - 10.1021/acs.cgd.6b01754
UR - https://doi.org/10.1021/acs.cgd.6b01754
TI - H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes
T2 - Crystal Growth and Design
AU - Ivanov, Daniil M
AU - Kinzhalov, M. A.
AU - Novikov, Alexander S.
AU - Ananyev, Ivan V
AU - Romanova, Anna A
AU - Boyarskiy, Vadim P
AU - Haukka, Matti
AU - Kukushkin, Vadim Yu.
PY - 2017
DA - 2017/02/01
PB - American Chemical Society (ACS)
SP - 1353-1362
IS - 3
VL - 17
SN - 1528-7483
SN - 1528-7505
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2017_Ivanov,
author = {Daniil M Ivanov and M. A. Kinzhalov and Alexander S. Novikov and Ivan V Ananyev and Anna A Romanova and Vadim P Boyarskiy and Matti Haukka and Vadim Yu. Kukushkin},
title = {H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes},
journal = {Crystal Growth and Design},
year = {2017},
volume = {17},
publisher = {American Chemical Society (ACS)},
month = {feb},
url = {https://doi.org/10.1021/acs.cgd.6b01754},
number = {3},
pages = {1353--1362},
doi = {10.1021/acs.cgd.6b01754}
}
MLA
Cite this
MLA Copy
Ivanov, Daniil M., et al. “H2C(X)–X···X– (X = Cl, Br) Halogen Bonding of Dihalomethanes.” Crystal Growth and Design, vol. 17, no. 3, Feb. 2017, pp. 1353-1362. https://doi.org/10.1021/acs.cgd.6b01754.