Chemistry of Materials, volume 27, issue 15, pages 5407-5416

Stable Interface Formation between TiS₂ and LiBH₄ in Bulk-Type All-Solid-State Lithium Batteries

Atsushi Unemoto ¹

Tamio Ikeshoji ^{1, 2}

Syun Yasaku ²

Motoaki Matsuo ²

Vitalie Stavila ³

Terrence John Udovic ⁴

Shin-ichi Orimo ^{1, 2}

Hide authors affiliations Show authors affiliations: 4 affiliations

WPI−Advanced Institute for Materials Research (WPI−AIMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, Japan |

Institute for Materials Research, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577, Japan |

Energy Nanomaterials, Sandia National Laboratories, Livermore, California 94551, United States |

⁴

NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899-6102, United States |

Publication type: Journal Article

Publication date: 2015-07-28

American Chemical Society (ACS)

Journal: Chemistry of Materials

Quartile SCImago

Quartile WOS

Impact factor: 8.6

ISSN: 08974756, 15205002

DOI: 10.1021/acs.chemmater.5b02110

Copy DOI

Materials Chemistry

General Chemistry

General Chemical Engineering

Abstract

In this study, we assembled a bulk-type all-solid-state battery comprised of a TiS2 positive electrode, LiBH4 electrolyte, and Li negative electrode. Our battery retained high capacity over 300 discharge–charge cycles when operated at 393 K and 0.2 C. The second discharge capacity was as high as 205 mAh g–1, corresponding to a TiS2 utilization ratio of 85%. The 300th discharge capacity remained as high as 180 mAh g–1 with nearly 100% Coulombic efficiency from the second cycle. Negligible impact of the exposure of LiBH4 to atmospheric-pressure oxygen on battery cycle life was also confirmed. To investigate the origin of the cycle durability for this bulk-type all-solid-state TiS2/Li battery, electrochemical measurements, thermogravimetry coupled with gas composition analysis, powder X-ray diffraction measurements, and first-principles molecular dynamics simulations were carried out. Chemical and/or electrochemical oxidation of LiBH4 occurred at the TiS2 surface at the battery operating temperature of 393 K...

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	1 2 3 4 5 6 7
Journal of Alloys and Compounds	Journal of Alloys and Compounds, 7, 5.88% Journal of Alloys and Compounds 7 publications, 5.88%
ACS applied materials & interfaces	ACS applied materials & interfaces, 6, 5.04% ACS applied materials & interfaces 6 publications, 5.04%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 4, 3.36% Journal of Solid State Electrochemistry 4 publications, 3.36%
Electrochimica Acta	Electrochimica Acta, 4, 3.36% Electrochimica Acta 4 publications, 3.36%
ACS Applied Energy Materials	ACS Applied Energy Materials, 4, 3.36% ACS Applied Energy Materials 4 publications, 3.36%
Materials Transactions	Materials Transactions, 3, 2.52% Materials Transactions 3 publications, 2.52%
Energy Storage Materials	Energy Storage Materials, 3, 2.52% Energy Storage Materials 3 publications, 2.52%
Journal of Energy Chemistry	Journal of Energy Chemistry, 3, 2.52% Journal of Energy Chemistry 3 publications, 2.52%
Solid State Ionics	Solid State Ionics, 3, 2.52% Solid State Ionics 3 publications, 2.52%
Advanced Materials	Advanced Materials, 3, 2.52% Advanced Materials 3 publications, 2.52%
Chemistry of Materials	Chemistry of Materials, 3, 2.52% Chemistry of Materials 3 publications, 2.52%
ACS Energy Letters	ACS Energy Letters, 3, 2.52% ACS Energy Letters 3 publications, 2.52%
Materia Japan	Materia Japan, 2, 1.68% Materia Japan 2 publications, 1.68%
Molecules	Molecules, 2, 1.68% Molecules 2 publications, 1.68%
Materials	Materials, 2, 1.68% Materials 2 publications, 1.68%
Journal of Materials Science and Technology	Journal of Materials Science and Technology, 2, 1.68% Journal of Materials Science and Technology 2 publications, 1.68%
Nature Communications	Nature Communications, 2, 1.68% Nature Communications 2 publications, 1.68%
Chemical Engineering Journal	Chemical Engineering Journal, 2, 1.68% Chemical Engineering Journal 2 publications, 1.68%
Advanced Energy Materials	Advanced Energy Materials, 2, 1.68% Advanced Energy Materials 2 publications, 1.68%
Advanced Functional Materials	Advanced Functional Materials, 2, 1.68% Advanced Functional Materials 2 publications, 1.68%
Inorganic Chemistry	Inorganic Chemistry, 2, 1.68% Inorganic Chemistry 2 publications, 1.68%
Journal of the American Chemical Society	Journal of the American Chemical Society, 2, 1.68% Journal of the American Chemical Society 2 publications, 1.68%
Journal of Physical Chemistry Letters	Journal of Physical Chemistry Letters, 2, 1.68% Journal of Physical Chemistry Letters 2 publications, 1.68%
Chemical Society Reviews	Chemical Society Reviews, 2, 1.68% Chemical Society Reviews 2 publications, 1.68%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 2, 1.68% Journal of Materials Chemistry A 2 publications, 1.68%
Applied Physics Letters	Applied Physics Letters, 1, 0.84% Applied Physics Letters 1 publication, 0.84%
Electrochemistry	Electrochemistry, 1, 0.84% Electrochemistry 1 publication, 0.84%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 1, 0.84% Journal of Physical Chemistry C 1 publication, 0.84%
Nippon Kinzoku Gakkaishi/Journal of the Japan Institute of Metals	Nippon Kinzoku Gakkaishi/Journal of the Japan Institute of Metals, 1, 0.84% Nippon Kinzoku Gakkaishi/Journal of the Japan Institute of Metals 1 publication, 0.84%
	1 2 3 4 5 6 7

Citations by publishers

	5 10 15 20 25 30 35
Elsevier	Elsevier, 32, 26.89% Elsevier 32 publications, 26.89%
American Chemical Society (ACS)	American Chemical Society (ACS), 26, 21.85% American Chemical Society (ACS) 26 publications, 21.85%
Wiley	Wiley, 15, 12.61% Wiley 15 publications, 12.61%
Springer Nature	Springer Nature, 13, 10.92% Springer Nature 13 publications, 10.92%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 12, 10.08% Royal Society of Chemistry (RSC) 12 publications, 10.08%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 7, 5.88% Multidisciplinary Digital Publishing Institute (MDPI) 7 publications, 5.88%
Japan Institute of Metals and Materials	Japan Institute of Metals and Materials, 5, 4.2% Japan Institute of Metals and Materials 5 publications, 4.2%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 1, 0.84% American Institute of Physics (AIP) 1 publication, 0.84%
The Electrochemical Society of Japan	The Electrochemical Society of Japan, 1, 0.84% The Electrochemical Society of Japan 1 publication, 0.84%
Nippon Kinzoku Gakkai	Nippon Kinzoku Gakkai, 1, 0.84% Nippon Kinzoku Gakkai 1 publication, 0.84%
Cambridge University Press	Cambridge University Press, 1, 0.84% Cambridge University Press 1 publication, 0.84%
Pleiades Publishing	Pleiades Publishing, 1, 0.84% Pleiades Publishing 1 publication, 0.84%
Walter de Gruyter	Walter de Gruyter, 1, 0.84% Walter de Gruyter 1 publication, 0.84%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.84% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.84%
	5 10 15 20 25 30 35

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Unemoto A. et al. Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries // Chemistry of Materials. 2015. Vol. 27. No. 15. pp. 5407-5416.

GOST all authors (up to 50) Copy

Unemoto A., Ikeshoji T., Yasaku S., Matsuo M., Stavila V., Udovic T. J., Orimo S. Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries // Chemistry of Materials. 2015. Vol. 27. No. 15. pp. 5407-5416.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acs.chemmater.5b02110

UR - https://doi.org/10.1021/acs.chemmater.5b02110

TI - Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries

T2 - Chemistry of Materials

AU - Unemoto, Atsushi

AU - Yasaku, Syun

AU - Matsuo, Motoaki

AU - Ikeshoji, Tamio

AU - Stavila, Vitalie

AU - Udovic, Terrence John

AU - Orimo, Shin-ichi

PY - 2015

DA - 2015/07/28 00:00:00

PB - American Chemical Society (ACS)

SP - 5407-5416

IS - 15

VL - 27

SN - 0897-4756

SN - 1520-5002

ER -

BibTex |

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BibTex Copy

@article{2015_Unemoto,

author = {Atsushi Unemoto and Syun Yasaku and Motoaki Matsuo and Tamio Ikeshoji and Vitalie Stavila and Terrence John Udovic and Shin-ichi Orimo},

title = {Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries},

journal = {Chemistry of Materials},

year = {2015},

volume = {27},

publisher = {American Chemical Society (ACS)},

month = {jul},

url = {https://doi.org/10.1021/acs.chemmater.5b02110},

number = {15},

pages = {5407--5416},

doi = {10.1021/acs.chemmater.5b02110}

}

MLA

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MLA Copy

Unemoto, Atsushi, et al. “Stable Interface Formation between TiS2 and LiBH4 in Bulk-Type All-Solid-State Lithium Batteries.” Chemistry of Materials, vol. 27, no. 15, Jul. 2015, pp. 5407-5416. https://doi.org/10.1021/acs.chemmater.5b02110.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Chemistry of Materials

Quartile SCImago

Quartile WOS

Impact factor

8.6

ISSN

08974756 (Print)
15205002 (Electronic)