Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure
Mingyue Chen
1
,
Zhiguo Xia
1
,
Maxim S. Molokeev
2, 3, 4
,
Chun Che Lin
5
,
Chaochin Su
5
,
Yu-Liang Chuang
6
,
2
Тип публикации: Journal Article
Дата публикации: 2017-08-18
scimago Q1
wos Q1
БС1
SJR: 2.065
CiteScore: 12.0
Impact factor: 7.0
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Краткое описание
Eu2+ local environments in various crystallographic sites enable the different distributions of the emission and excitation energies and then realize the photoluminescence tuning of the Eu2+ doped solid state phosphors. Herein we report the Eu2+-doped Ca10M(PO4)7 (M = Li, Na, and K) phosphors with β-Ca3(PO4)2-type structure, in which there are five cation crystallographic sites, and the phosphors show a color tuning from bluish-violet to blue and yellow with the variation of M ions. The difference in decay rate monitored at selected wavelengths is related to multiple luminescent centers in Ca10M(PO4)7:Eu2+, and the occupied rates of Eu2+ in Ca(1), Ca(2), Ca(3), Na(4), and Ca(5) sites from Rietveld refinements using synchrotron power diffraction data confirm that Eu2+ enters into four cation sites except for Ca(5). Since the average bond lengths d(Ca–O) remain invariable in the Ca10M(PO4)7:Eu2+, the drastic changes of bond lengths d(M–O) and Eu2+ emission depending on the variation from Li to Na and K can ...
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Chen M. et al. Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure // Chemistry of Materials. 2017. Vol. 29. No. 17. pp. 7563-7570.
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Chen M., Xia Z., Molokeev M. S., Lin C. C., Su C., Chuang Y., Liu Q. L. Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure // Chemistry of Materials. 2017. Vol. 29. No. 17. pp. 7563-7570.
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TY - JOUR
DO - 10.1021/acs.chemmater.7b02724
UR - https://doi.org/10.1021/acs.chemmater.7b02724
TI - Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure
T2 - Chemistry of Materials
AU - Chen, Mingyue
AU - Xia, Zhiguo
AU - Molokeev, Maxim S.
AU - Lin, Chun Che
AU - Su, Chaochin
AU - Chuang, Yu-Liang
AU - Liu, Quan Lin
PY - 2017
DA - 2017/08/18
PB - American Chemical Society (ACS)
SP - 7563-7570
IS - 17
VL - 29
SN - 0897-4756
SN - 1520-5002
ER -
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@article{2017_Chen,
author = {Mingyue Chen and Zhiguo Xia and Maxim S. Molokeev and Chun Che Lin and Chaochin Su and Yu-Liang Chuang and Quan Lin Liu},
title = {Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure},
journal = {Chemistry of Materials},
year = {2017},
volume = {29},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.chemmater.7b02724},
number = {17},
pages = {7563--7570},
doi = {10.1021/acs.chemmater.7b02724}
}
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MLA
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Chen, Mingyue, et al. “Probing Eu2+ luminescence from different crystallographic sites in Ca10M(PO4)7:Eu2+ (M = Li, Na and K) with β-Ca3(PO4)2-type structure.” Chemistry of Materials, vol. 29, no. 17, Aug. 2017, pp. 7563-7570. https://doi.org/10.1021/acs.chemmater.7b02724.
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