Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex
Тип публикации: Journal Article
Дата публикации: 2017-10-06
scimago Q1
Tоп 10% SciMago
wos Q1
white level БС1
SJR: 2.065
CiteScore: 12
Impact factor: 7
ISSN: 08974756, 15205002
Materials Chemistry
General Chemistry
General Chemical Engineering
Краткое описание
Li+- and Na+-conducting thiophosphates have attracted much interest because of their intrinsically high ionic conductivities and the possibility to be employed in solid-state batteries. Inspired by the recent finding of the influence of changing lattice vibrations and induced lattice softening on the ionic transport of Li+-conducting electrolytes, here we explore this effect in the Na+ conductor Na3PS4–xSex. Ultrasonic speed of sound measurements are used to monitor a changing lattice stiffness and Debye frequencies. The changes in the lattice dynamics are complemented by X-ray diffraction and electrochemical impedance spectroscopy. With systematic alteration of the polarizability of the anion framework, a softening of the lattice can be observed that leads to a reduction of the activation barrier for migration as well as a decreased Arrhenius prefactor. This work shows that, similar to Li+ transport, the softening of the average vibrational frequencies of the lattice has a tremendous effect on Na+-ionic ...
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Krauskopf T. et al. Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex // Chemistry of Materials. 2017. Vol. 29. No. 20. pp. 8859-8869.
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Krauskopf T., Pompe C., Kraft M. A., Zeier W. G. Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex // Chemistry of Materials. 2017. Vol. 29. No. 20. pp. 8859-8869.
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TY - JOUR
DO - 10.1021/acs.chemmater.7b03474
UR - https://doi.org/10.1021/acs.chemmater.7b03474
TI - Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex
T2 - Chemistry of Materials
AU - Krauskopf, Thorben
AU - Pompe, Constantin
AU - Kraft, Marvin A
AU - Zeier, Wolfgang G.
PY - 2017
DA - 2017/10/06
PB - American Chemical Society (ACS)
SP - 8859-8869
IS - 20
VL - 29
SN - 0897-4756
SN - 1520-5002
ER -
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BibTex (до 50 авторов)
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@article{2017_Krauskopf,
author = {Thorben Krauskopf and Constantin Pompe and Marvin A Kraft and Wolfgang G. Zeier},
title = {Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex},
journal = {Chemistry of Materials},
year = {2017},
volume = {29},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.chemmater.7b03474},
number = {20},
pages = {8859--8869},
doi = {10.1021/acs.chemmater.7b03474}
}
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MLA
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Krauskopf, Thorben, et al. “Influence of Lattice Dynamics on Na+ Transport in the Solid Electrolyte Na3PS4–xSex.” Chemistry of Materials, vol. 29, no. 20, Oct. 2017, pp. 8859-8869. https://doi.org/10.1021/acs.chemmater.7b03474.
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