Chemical Reviews, volume 122, issue 3, pages 3763-3819

Antiperovskite Electrolytes for Solid-State Batteries

Wei Xia ^{1, 2}

Yang Zhao ¹

Feipeng Zhao ¹

Keegan Adair ¹

Ruo Zhao ²

Shuai Li ²

Yusheng Zhao ³

Yusheng Zhao ²

Xueliang Andy Sun ¹

Hide authors affiliations Show authors affiliations: 3 affiliations

Department of Mechanical and Materials Engineering, University of Western Ontario, London, OntarioN6A 5B9, Canada |

Shenzhen Key Laboratory of Solid State Batteries, Guangdong Provincial Key Laboratory of Energy Materials for Electric Power, Academy for Advanced Interdisciplinary Studies, Southern University of Science and Technology, Shenzhen518055, China |

Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials, School of Materials Science and Engineering, Peking University, Beijing100871, China |

Publication type: Journal Article

Publication date: 2022-01-11

American Chemical Society (ACS)

Journal: Chemical Reviews

Quartile SCImago

Quartile WOS

Impact factor: 62.1

ISSN: 00092665, 15206890

DOI: 10.1021/acs.chemrev.1c00594

Copy DOI

General Chemistry

Abstract

Solid-state batteries have fascinated the research community over the past decade, largely due to their improved safety properties and potential for high-energy density. Searching for fast ion conductors with sufficient electrochemical and chemical stabilities is at the heart of solid-state battery research and applications. Recently, significant progress has been made in solid-state electrolyte development. Sulfide-, oxide-, and halide-based electrolytes have been able to achieve high ionic conductivities of more than 10-3 S/cm at room temperature, which are comparable to liquid-based electrolytes. However, their stability toward Li metal anodes poses significant challenges for these electrolytes. The existence of non-Li cations that can be reduced by Li metal in these electrolytes hinders the application of Li anode and therefore poses an obstacle toward achieving high-energy density. The finding of antiperovskites as ionic conductors in recent years has demonstrated a new and exciting solution. These materials, mainly constructed from Li (or Na), O, and Cl (or Br), are lightweight and electrochemically stable toward metallic Li and possess promising ionic conductivity. Because of the structural flexibility and tunability, antiperovskite electrolytes are excellent candidates for solid-state battery applications, and researchers are still exploring the relationship between their structure and ion diffusion behavior. Herein, the recent progress of antiperovskites for solid-state batteries is reviewed, and the strategies to tune the ionic conductivity by structural manipulation are summarized. Major challenges and future directions are discussed to facilitate the development of antiperovskite-based solid-state batteries.

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Citations by journals

	1 2 3 4 5 6 7 8
Advanced Energy Materials	Advanced Energy Materials, 8, 6.2% Advanced Energy Materials 8 publications, 6.2%
Advanced Functional Materials	Advanced Functional Materials, 5, 3.88% Advanced Functional Materials 5 publications, 3.88%
Journal of Materials Chemistry A	Journal of Materials Chemistry A, 5, 3.88% Journal of Materials Chemistry A 5 publications, 3.88%
Advanced Materials	Advanced Materials, 4, 3.1% Advanced Materials 4 publications, 3.1%
Chemistry of Materials	Chemistry of Materials, 4, 3.1% Chemistry of Materials 4 publications, 3.1%
Journal of Physical Chemistry C	Journal of Physical Chemistry C, 4, 3.1% Journal of Physical Chemistry C 4 publications, 3.1%
Small	Small, 4, 3.1% Small 4 publications, 3.1%
ACS applied materials & interfaces	ACS applied materials & interfaces, 4, 3.1% ACS applied materials & interfaces 4 publications, 3.1%
Energy Storage Materials	Energy Storage Materials, 4, 3.1% Energy Storage Materials 4 publications, 3.1%
Batteries	Batteries, 3, 2.33% Batteries 3 publications, 2.33%
Energy and Environmental Science	Energy and Environmental Science, 3, 2.33% Energy and Environmental Science 3 publications, 2.33%
Progress in Materials Science	Progress in Materials Science, 3, 2.33% Progress in Materials Science 3 publications, 2.33%
Journal of the American Chemical Society	Journal of the American Chemical Society, 3, 2.33% Journal of the American Chemical Society 3 publications, 2.33%
Chinese Chemical Letters	Chinese Chemical Letters, 3, 2.33% Chinese Chemical Letters 3 publications, 2.33%
Journal of Solid State Electrochemistry	Journal of Solid State Electrochemistry, 2, 1.55% Journal of Solid State Electrochemistry 2 publications, 1.55%
Jiegou Huaxue	Jiegou Huaxue, 2, 1.55% Jiegou Huaxue 2 publications, 1.55%
Journal of Solid State Chemistry	Journal of Solid State Chemistry, 2, 1.55% Journal of Solid State Chemistry 2 publications, 1.55%
Journal of Energy Chemistry	Journal of Energy Chemistry, 2, 1.55% Journal of Energy Chemistry 2 publications, 1.55%
Batteries & Supercaps	Batteries & Supercaps, 2, 1.55% Batteries & Supercaps 2 publications, 1.55%
ACS Applied Energy Materials	ACS Applied Energy Materials, 2, 1.55% ACS Applied Energy Materials 2 publications, 1.55%
RSC Advances	RSC Advances, 2, 1.55% RSC Advances 2 publications, 1.55%
Interdisciplinary Materials	Interdisciplinary Materials, 2, 1.55% Interdisciplinary Materials 2 publications, 1.55%
Advanced Science	Advanced Science, 2, 1.55% Advanced Science 2 publications, 1.55%
Journal of Colloid and Interface Science	Journal of Colloid and Interface Science, 2, 1.55% Journal of Colloid and Interface Science 2 publications, 1.55%
ACS Nano	ACS Nano, 2, 1.55% ACS Nano 2 publications, 1.55%
Materials Horizons	Materials Horizons, 1, 0.78% Materials Horizons 1 publication, 0.78%
Journal of the Electrochemical Society	Journal of the Electrochemical Society, 1, 0.78% Journal of the Electrochemical Society 1 publication, 0.78%
Frontiers in Chemistry	Frontiers in Chemistry, 1, 0.78% Frontiers in Chemistry 1 publication, 0.78%
Materials	Materials, 1, 0.78% Materials 1 publication, 0.78%
	1 2 3 4 5 6 7 8

Citations by publishers

	5 10 15 20 25 30 35 40
Wiley	Wiley, 37, 28.68% Wiley 37 publications, 28.68%
Elsevier	Elsevier, 33, 25.58% Elsevier 33 publications, 25.58%
American Chemical Society (ACS)	American Chemical Society (ACS), 21, 16.28% American Chemical Society (ACS) 21 publications, 16.28%
Royal Society of Chemistry (RSC)	Royal Society of Chemistry (RSC), 13, 10.08% Royal Society of Chemistry (RSC) 13 publications, 10.08%
Springer Nature	Springer Nature, 7, 5.43% Springer Nature 7 publications, 5.43%
Multidisciplinary Digital Publishing Institute (MDPI)	Multidisciplinary Digital Publishing Institute (MDPI), 4, 3.1% Multidisciplinary Digital Publishing Institute (MDPI) 4 publications, 3.1%
Chinese Academy of Sciences	Chinese Academy of Sciences, 2, 1.55% Chinese Academy of Sciences 2 publications, 1.55%
American Institute of Physics (AIP)	American Institute of Physics (AIP), 2, 1.55% American Institute of Physics (AIP) 2 publications, 1.55%
The Electrochemical Society	The Electrochemical Society, 1, 0.78% The Electrochemical Society 1 publication, 0.78%
Frontiers Media S.A.	Frontiers Media S.A., 1, 0.78% Frontiers Media S.A. 1 publication, 0.78%
IOP Publishing	IOP Publishing, 1, 0.78% IOP Publishing 1 publication, 0.78%
American Association for the Advancement of Science (AAAS)	American Association for the Advancement of Science (AAAS), 1, 0.78% American Association for the Advancement of Science (AAAS) 1 publication, 0.78%
Walter de Gruyter	Walter de Gruyter, 1, 0.78% Walter de Gruyter 1 publication, 0.78%
Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii	Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii, 1, 0.78% Autonomous Non-profit Organization Editorial Board of the journal Uspekhi Khimii 1 publication, 0.78%
	5 10 15 20 25 30 35 40

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Xia W. et al. Antiperovskite Electrolytes for Solid-State Batteries // Chemical Reviews. 2022. Vol. 122. No. 3. pp. 3763-3819.

GOST all authors (up to 50) Copy

Xia W., Zhao Y., Zhao F., Adair K., Zhao R., Li S., Zhao Y., Zhao Y., Sun X. A. Antiperovskite Electrolytes for Solid-State Batteries // Chemical Reviews. 2022. Vol. 122. No. 3. pp. 3763-3819.

RIS |

Cite this

RIS Copy

TY - JOUR

DO - 10.1021/acs.chemrev.1c00594

UR - https://doi.org/10.1021/acs.chemrev.1c00594

TI - Antiperovskite Electrolytes for Solid-State Batteries

T2 - Chemical Reviews

AU - Xia, Wei

AU - Zhao, Feipeng

AU - Adair, Keegan

AU - Zhao, Ruo

AU - Li, Shuai

AU - Zhao, Yusheng

AU - Zhao, Yang

AU - Zhao, Yusheng

AU - Sun, Xueliang Andy

PY - 2022

DA - 2022/01/11 00:00:00

PB - American Chemical Society (ACS)

SP - 3763-3819

IS - 3

VL - 122

SN - 0009-2665

SN - 1520-6890

ER -

BibTex |

Cite this

BibTex Copy

@article{2022_Xia,

author = {Wei Xia and Feipeng Zhao and Keegan Adair and Ruo Zhao and Shuai Li and Yusheng Zhao and Yang Zhao and Yusheng Zhao and Xueliang Andy Sun},

title = {Antiperovskite Electrolytes for Solid-State Batteries},

journal = {Chemical Reviews},

year = {2022},

volume = {122},

publisher = {American Chemical Society (ACS)},

month = {jan},

url = {https://doi.org/10.1021/acs.chemrev.1c00594},

number = {3},

pages = {3763--3819},

doi = {10.1021/acs.chemrev.1c00594}

}

MLA

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MLA Copy

Xia, Wei, et al. “Antiperovskite Electrolytes for Solid-State Batteries.” Chemical Reviews, vol. 122, no. 3, Jan. 2022, pp. 3763-3819. https://doi.org/10.1021/acs.chemrev.1c00594.

Found error?

Publisher

American Chemical Society (ACS)

Journal

Chemical Reviews

Quartile SCImago

Quartile WOS

Impact factor

62.1

ISSN

00092665 (Print)
15206890 (Electronic)