Chemical Reviews, volume 116, issue 21, pages 12865-12919
Electronic Processes within Quantum Dot-Molecule Complexes
Publication type: Journal Article
Publication date: 2016-08-08
Journal:
Chemical Reviews
Quartile SCImago
Q1
Quartile WOS
Q1
Impact factor: 62.1
ISSN: 00092665, 15206890
General Chemistry
Abstract
The subject of this review is the colloidal quantum dot (QD) and specifically the interaction of the QD with proximate molecules. It covers various functions of these molecules, including (i) ligands for the QDs, coupled electronically or vibrationally to localized surface states or to the delocalized states of the QD core, (ii) energy or electron donors or acceptors for the QDs, and (iii) structural components of QD assemblies that dictate QD-QD or QD-molecule interactions. Research on interactions of ligands with colloidal QDs has revealed that ligands determine not only the excited state dynamics of the QD but also, in some cases, its ground state electronic structure. Specifically, the article discusses (i) measurement of the electronic structure of colloidal QDs and the influence of their surface chemistry, in particular, dipolar ligands and exciton-delocalizing ligands, on their electronic energies; (ii) the role of molecules in interfacial electron and energy transfer processes involving QDs, including electron-to-vibrational energy transfer and the use of the ligand shell of a QD as a semipermeable membrane that gates its redox activity; and (iii) a particular application of colloidal QDs, photoredox catalysis, which exploits the combination of the electronic structure of the QD core and the chemistry at its surface to use the energy of the QD excited state to drive chemical reactions.
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Harris R. D. et al. Electronic Processes within Quantum Dot-Molecule Complexes // Chemical Reviews. 2016. Vol. 116. No. 21. pp. 12865-12919.
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Harris R. D., Bettis Homan S., Kodaimati M., He C., Nepomnyashchii A. B., Swenson N. K., Lian S., Calzada R., Weiss E. A. Electronic Processes within Quantum Dot-Molecule Complexes // Chemical Reviews. 2016. Vol. 116. No. 21. pp. 12865-12919.
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TY - JOUR
DO - 10.1021/acs.chemrev.6b00102
UR - https://doi.org/10.1021/acs.chemrev.6b00102
TI - Electronic Processes within Quantum Dot-Molecule Complexes
T2 - Chemical Reviews
AU - Harris, Rachel D
AU - Bettis Homan, Stephanie
AU - Kodaimati, Mohamad
AU - Nepomnyashchii, Alexander B.
AU - Swenson, Nathaniel K
AU - Lian, Shichen
AU - Calzada, Raul
AU - He, Chen
AU - Weiss, Emily A.
PY - 2016
DA - 2016/08/08 00:00:00
PB - American Chemical Society (ACS)
SP - 12865-12919
IS - 21
VL - 116
SN - 0009-2665
SN - 1520-6890
ER -
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@article{2016_Harris,
author = {Rachel D Harris and Stephanie Bettis Homan and Mohamad Kodaimati and Alexander B. Nepomnyashchii and Nathaniel K Swenson and Shichen Lian and Raul Calzada and Chen He and Emily A. Weiss},
title = {Electronic Processes within Quantum Dot-Molecule Complexes},
journal = {Chemical Reviews},
year = {2016},
volume = {116},
publisher = {American Chemical Society (ACS)},
month = {aug},
url = {https://doi.org/10.1021/acs.chemrev.6b00102},
number = {21},
pages = {12865--12919},
doi = {10.1021/acs.chemrev.6b00102}
}
Cite this
MLA
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Harris, Rachel D., et al. “Electronic Processes within Quantum Dot-Molecule Complexes.” Chemical Reviews, vol. 116, no. 21, Aug. 2016, pp. 12865-12919. https://doi.org/10.1021/acs.chemrev.6b00102.