Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections
Chengdong Yuan
1
,
Aleksey A. Eskin
1
,
Ruslan N Nagrimanov
1
,
Mustafa Versan Kok
2
,
Igor S Afanasiev
3
,
Gennadii D Fedorchenko
3
,
Elena V Kopylova
3
3
JSC Zabubezhneft, Moscow, 101990, Russia
|
Тип публикации: Journal Article
Дата публикации: 2017-12-15
scimago Q1
wos Q1
БС1
SJR: 1.124
CiteScore: 9.5
Impact factor: 5.3
ISSN: 08870624, 15205029
General Chemical Engineering
Energy Engineering and Power Technology
Fuel Technology
Краткое описание
This research is intended to reveal the difference and connection of oxidation behavior between crude oil and its SARA fractions. Thermogravimetry (TG) and differential scanning calorimetry (DSC) techniques were used to characterize oxidation behavior. The results showed that the oxidation behavior of individual SARA components exhibited an obvious difference. Saturates showed a weak high-temperature oxidation (HTO) region. Asphaltenes generated more heat in HTO than in the low-temperature oxidation (LTO) region. Aromatics showed intense exothermic activity in both LTO and HTO regions. Heat release and mass loss showed a good correspondence in the HTO region for all SARA fractions, which means heat release and mass loss were caused by the same reaction mechanism that is believed to be the coke combustion as it is the only significant reaction in the HTO region. However, the good correspondence did not exist in the LTO interval where the reactions are more complicated and a multiple-step mechanism should b...
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Yuan C. et al. Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections // Energy & Fuels. 2017. Vol. 32. No. 1. pp. 801-808.
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Yuan C., Varfolomeev M. A., Emelianov D. A., Eskin A. A., Nagrimanov R. N., Kok M. V., Afanasiev I. S., Fedorchenko G. D., Kopylova E. V. Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections // Energy & Fuels. 2017. Vol. 32. No. 1. pp. 801-808.
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TY - JOUR
DO - 10.1021/acs.energyfuels.7b02377
UR - https://doi.org/10.1021/acs.energyfuels.7b02377
TI - Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections
T2 - Energy & Fuels
AU - Yuan, Chengdong
AU - Varfolomeev, Mikhail A.
AU - Emelianov, Dmitrii A
AU - Eskin, Aleksey A.
AU - Nagrimanov, Ruslan N
AU - Kok, Mustafa Versan
AU - Afanasiev, Igor S
AU - Fedorchenko, Gennadii D
AU - Kopylova, Elena V
PY - 2017
DA - 2017/12/15
PB - American Chemical Society (ACS)
SP - 801-808
IS - 1
VL - 32
SN - 0887-0624
SN - 1520-5029
ER -
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@article{2017_Yuan,
author = {Chengdong Yuan and Mikhail A. Varfolomeev and Dmitrii A Emelianov and Aleksey A. Eskin and Ruslan N Nagrimanov and Mustafa Versan Kok and Igor S Afanasiev and Gennadii D Fedorchenko and Elena V Kopylova},
title = {Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections},
journal = {Energy & Fuels},
year = {2017},
volume = {32},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.energyfuels.7b02377},
number = {1},
pages = {801--808},
doi = {10.1021/acs.energyfuels.7b02377}
}
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MLA
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Yuan, Chengdong, et al. “Oxidation Behavior of Light Crude Oil and Its SARA Fractions Characterized by TG and DSC Techniques: Differences and Connections.” Energy & Fuels, vol. 32, no. 1, Dec. 2017, pp. 801-808. https://doi.org/10.1021/acs.energyfuels.7b02377.