Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity
Zhiwei Huang
1, 2
,
Kong-qiu Hu
3
,
Lei Mei
3
,
Cong Zhi Wang
3
,
Yan-Mei Chen
1
,
Wang Suo Wu
2
,
Zhi-Fang Chai
1, 3
,
Publication type: Journal Article
Publication date: 2020-12-31
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
33382238
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The stability of many MOFs is not satisfactory, which severely limits the exploration of their potential applications. Given this, we have proposed a strategy to improve the stability of MOFs by introducing alkali metal K+ capable of coordinating with metal nodes, which finally induces the interpenetrating uranyl-porphyrin framework to connect as a whole (IHEP-9). The stability experiments reveal that the IHEP-9 has good thermal stability up to 400 °C and can maintain its crystalline state in the aqueous solution with pH ranging from 2 to 11. The catalytic activity of IHEP-9 as a heterogeneous photocatalyst for CO2 cycloaddition under the driving of visible light at room temperature is also demonstrated. This induced interpenetration and fixation method may be promising for the fabrication of more functional MOFs with improved structural stability.
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62
Total citations:
62
Citations from 2024:
25
(40.32%)
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GOST
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Huang Z. et al. Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity // Inorganic Chemistry. 2020. Vol. 60. No. 2. pp. 651-659.
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Huang Z., Hu K., Mei L., Wang C. Z., Chen Y., Wu W. S., Chai Z., Shi W. Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity // Inorganic Chemistry. 2020. Vol. 60. No. 2. pp. 651-659.
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TY - JOUR
DO - 10.1021/acs.inorgchem.0c02473
UR - https://doi.org/10.1021/acs.inorgchem.0c02473
TI - Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity
T2 - Inorganic Chemistry
AU - Huang, Zhiwei
AU - Hu, Kong-qiu
AU - Mei, Lei
AU - Wang, Cong Zhi
AU - Chen, Yan-Mei
AU - Wu, Wang Suo
AU - Chai, Zhi-Fang
AU - Shi, Wei-Qun
PY - 2020
DA - 2020/12/31
PB - American Chemical Society (ACS)
SP - 651-659
IS - 2
VL - 60
PMID - 33382238
SN - 0020-1669
SN - 1520-510X
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2020_Huang,
author = {Zhiwei Huang and Kong-qiu Hu and Lei Mei and Cong Zhi Wang and Yan-Mei Chen and Wang Suo Wu and Zhi-Fang Chai and Wei-Qun Shi},
title = {Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity},
journal = {Inorganic Chemistry},
year = {2020},
volume = {60},
publisher = {American Chemical Society (ACS)},
month = {dec},
url = {https://doi.org/10.1021/acs.inorgchem.0c02473},
number = {2},
pages = {651--659},
doi = {10.1021/acs.inorgchem.0c02473}
}
Cite this
MLA
Copy
Huang, Zhiwei, et al. “Potassium Ions Induced Framework Interpenetration for Enhancing the Stability of Uranium-Based Porphyrin MOF with Visible-Light-Driven Photocatalytic Activity.” Inorganic Chemistry, vol. 60, no. 2, Dec. 2020, pp. 651-659. https://doi.org/10.1021/acs.inorgchem.0c02473.
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