Assembly of Heterometallic AuICu2 I2 Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine
Irina R Dayanova
1
,
Igor D Strelnik
1
,
Tatiana P Gerasimova
1
,
R. А. Fayzullin
1
,
Daut R. Islamov
1
,
Alina Saifina
1
,
Alina F Saifina
1
,
Elvira Musina
1
,
Publication type: Journal Article
Publication date: 2021-03-24
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
33759505
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
The row of metallocyclic dinuclear gold(I) complexes with cyclic diphosphines, namely, P-pyridylethyl-substituted 1,5-diaza-3,7-diphosphacyclooctanes, has been obtained. Further interaction of the dinuclear gold(I) complexes with copper(I) iodide gave the first examples of hexanuclear AuI/CuI complexes containing two unusual trinuclear AuICu2I2 fragments. The structures of di- and hexanuclear complexes were confirmed by NMR spectroscopy, ESI mass spectrometry, elemental analysis, and single-crystal X-ray diffraction. All of the obtained complexes are moderate emitters in the solid state. Dinuclear gold(I) complexes displayed a greenish emission with the maxima in the emission spectra at ca. 550 nm. The obtained hexanuclear heterobimetallic AuI/CuI complexes are triplet solid-state blue emitters with the maximum in the emission spectra at 463 and 484 nm. According to the TD-DFT calculations, the observed emission of all studied complexes had a triplet origin and was caused by the 3CC or 3(MLCT) T1 → S0 transitions for dinuclear and hexanuclear complexes, respectively.
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Dayanova I. R. et al. Assembly of Heterometallic AuICu2I2Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine // Inorganic Chemistry. 2021. Vol. 60. No. 7. pp. 5402-5411.
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Dayanova I. R., Shamsieva A. V., Strelnik I. D., Gerasimova T. I., Gerasimova T. P., Kolesnikov I. E., Fayzullin R. А., R. Islamov D., Saifina A., Saifina A. F., Musina E., Hey-Hawkins E., Karasik A. A. Assembly of Heterometallic AuICu2I2Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine // Inorganic Chemistry. 2021. Vol. 60. No. 7. pp. 5402-5411.
Cite this
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TY - JOUR
DO - 10.1021/acs.inorgchem.1c00442
UR - https://pubs.acs.org/doi/10.1021/acs.inorgchem.1c00442
TI - Assembly of Heterometallic AuICu2I2Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine
T2 - Inorganic Chemistry
AU - Dayanova, Irina R
AU - Shamsieva, Aliia V
AU - Strelnik, Igor D
AU - Gerasimova, Tatiana I.
AU - Gerasimova, Tatiana P
AU - Kolesnikov, Ilya E.
AU - Fayzullin, R. А.
AU - R. Islamov, Daut
AU - Saifina, Alina
AU - Saifina, Alina F
AU - Musina, Elvira
AU - Hey-Hawkins, Evamarie
AU - Karasik, Andrey A
PY - 2021
DA - 2021/03/24
PB - American Chemical Society (ACS)
SP - 5402-5411
IS - 7
VL - 60
PMID - 33759505
SN - 0020-1669
SN - 1520-510X
ER -
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BibTex (up to 50 authors)
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@article{2021_Dayanova,
author = {Irina R Dayanova and Aliia V Shamsieva and Igor D Strelnik and Tatiana I. Gerasimova and Tatiana P Gerasimova and Ilya E. Kolesnikov and R. А. Fayzullin and Daut R. Islamov and Alina Saifina and Alina F Saifina and Elvira Musina and Evamarie Hey-Hawkins and Andrey A Karasik},
title = {Assembly of Heterometallic AuICu2I2Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine},
journal = {Inorganic Chemistry},
year = {2021},
volume = {60},
publisher = {American Chemical Society (ACS)},
month = {mar},
url = {https://pubs.acs.org/doi/10.1021/acs.inorgchem.1c00442},
number = {7},
pages = {5402--5411},
doi = {10.1021/acs.inorgchem.1c00442}
}
Cite this
MLA
Copy
Dayanova, Irina R., et al. “Assembly of Heterometallic AuICu2I2Cores on the Scaffold of NPPN-Bridging Cyclic Bisphosphine.” Inorganic Chemistry, vol. 60, no. 7, Mar. 2021, pp. 5402-5411. https://pubs.acs.org/doi/10.1021/acs.inorgchem.1c00442.