Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework
1
Beamline
Division, Pohang Accelerator Laboratory, 80 Jigokro-127-beongil, Nam-gu Pohang, Gyungbuk 37673, Republic of Korea
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Publication type: Journal Article
Publication date: 2016-01-28
scimago Q1
wos Q1
SJR: 0.958
CiteScore: 7.4
Impact factor: 4.7
ISSN: 00201669, 1520510X
PubMed ID:
26819090
Inorganic Chemistry
Physical and Theoretical Chemistry
Abstract
Flexible metal-organic frameworks (MOFs) show the structural transition phenomena, gate opening and breathing, upon the input of external stimuli. These phenomena have significant implications in their adsorptive applications. In this work, we demonstrate the direct capture of these gate-opening and breathing phenomena, triggered by CO2 molecules, in a well-designed flexible MOF composed of rotational sites and molecular gates. Combining X-ray single crystallographic data of a flexible MOF during gate opening/closing and breathing with in situ X-ray powder diffraction results uncovered the origin of this flexibility. Furthermore, computational studies revealed the specific sites required to open these gates by interaction with CO2 molecules.
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Total citations:
99
Citations from 2025:
11
(11.11%)
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GOST
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Hyun S. M. et al. Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework // Inorganic Chemistry. 2016. Vol. 55. No. 4. pp. 1920-1925.
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Moon D. Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework // Inorganic Chemistry. 2016. Vol. 55. No. 4. pp. 1920-1925.
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TY - JOUR
DO - 10.1021/acs.inorgchem.5b02874
UR - https://doi.org/10.1021/acs.inorgchem.5b02874
TI - Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework
T2 - Inorganic Chemistry
AU - Moon, Dohyun
PY - 2016
DA - 2016/01/28
PB - American Chemical Society (ACS)
SP - 1920-1925
IS - 4
VL - 55
PMID - 26819090
SN - 0020-1669
SN - 1520-510X
ER -
Cite this
BibTex (up to 50 authors)
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@article{2016_Hyun,
author = {Dohyun Moon},
title = {Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework},
journal = {Inorganic Chemistry},
year = {2016},
volume = {55},
publisher = {American Chemical Society (ACS)},
month = {jan},
url = {https://doi.org/10.1021/acs.inorgchem.5b02874},
number = {4},
pages = {1920--1925},
doi = {10.1021/acs.inorgchem.5b02874}
}
Cite this
MLA
Copy
Hyun, Sung Min, et al. “Exploration of Gate-Opening and Breathing Phenomena in a Tailored Flexible Metal–Organic Framework.” Inorganic Chemistry, vol. 55, no. 4, Jan. 2016, pp. 1920-1925. https://doi.org/10.1021/acs.inorgchem.5b02874.