volume 84 issue 21 pages 13794-13806

Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines

Roman S Malykhin 1, 2
Aleksandr O Kokuev 1, 3
Valentin S Dorokhov 1, 3
Vladimir A Tartakovsky 1
Publication typeJournal Article
Publication date2019-10-09
scimago Q2
wos Q1
SJR0.737
CiteScore6.1
Impact factor3.6
ISSN00223263, 15206904
Organic Chemistry
Abstract
In this article, comprehensive studies on the nucleophilic chlorination and bromination of readily available six-membered cyclic nitronates (1,2-oxazine-N-oxides) are reported. Under optimized conditions (POCl3 or (COBr)2 with Hünig's base), 3-halo-substituted 1,2-oxazines, which are difficult to access by other routes, were obtained in good to high yields. The latter were shown to be convenient precursors to other 3-substituted 1,2-oxazine derivatives using Lewis/Brønsted acid-assisted substitution of the halide atom for C-, S-, and N-nucleophiles.
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Malykhin R. S. et al. Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines // Journal of Organic Chemistry. 2019. Vol. 84. No. 21. pp. 13794-13806.
GOST all authors (up to 50) Copy
Malykhin R. S., Kokuev A. O., Dorokhov V. S., Nelyubina Y. V., Tartakovsky V. A., Tabolin A. A., Ioffe S. L., Sukhorukov A. Yu. Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines // Journal of Organic Chemistry. 2019. Vol. 84. No. 21. pp. 13794-13806.
RIS |
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RIS Copy
TY - JOUR
DO - 10.1021/acs.joc.9b02010
UR - https://doi.org/10.1021/acs.joc.9b02010
TI - Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines
T2 - Journal of Organic Chemistry
AU - Malykhin, Roman S
AU - Kokuev, Aleksandr O
AU - Dorokhov, Valentin S
AU - Nelyubina, Yulia V.
AU - Tartakovsky, Vladimir A
AU - Tabolin, Andrey A
AU - Ioffe, Sema L.
AU - Sukhorukov, Alexey Yu
PY - 2019
DA - 2019/10/09
PB - American Chemical Society (ACS)
SP - 13794-13806
IS - 21
VL - 84
PMID - 31595751
SN - 0022-3263
SN - 1520-6904
ER -
BibTex |
Cite this
BibTex (up to 50 authors) Copy
@article{2019_Malykhin,
author = {Roman S Malykhin and Aleksandr O Kokuev and Valentin S Dorokhov and Yulia V. Nelyubina and Vladimir A Tartakovsky and Andrey A Tabolin and Sema L. Ioffe and Alexey Yu Sukhorukov},
title = {Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines},
journal = {Journal of Organic Chemistry},
year = {2019},
volume = {84},
publisher = {American Chemical Society (ACS)},
month = {oct},
url = {https://doi.org/10.1021/acs.joc.9b02010},
number = {21},
pages = {13794--13806},
doi = {10.1021/acs.joc.9b02010}
}
MLA
Cite this
MLA Copy
Malykhin, Roman S., et al. “Nucleophilic Halogenation of Cyclic Nitronates: A General Access to 3-Halo-1,2-Oxazines.” Journal of Organic Chemistry, vol. 84, no. 21, Oct. 2019, pp. 13794-13806. https://doi.org/10.1021/acs.joc.9b02010.