Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite
Publication type: Journal Article
Publication date: 2015-04-22
scimago Q1
wos Q3
SJR: 0.742
CiteScore: 5.3
Impact factor: 2.9
ISSN: 15206106, 15205207, 10895647
PubMed ID:
25867974
Materials Chemistry
Surfaces, Coatings and Films
Physical and Theoretical Chemistry
Abstract
The light-induced charge-transfer (CT) state in the composite of the conductive polymer poly(3-hexylthiophene) (P3HT) and the fullerene derivative [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) has been studied by electron spin echo (ESE) spectroscopy. The out-of-phase ESE signal corresponding to the spin-correlated radical pair P3HT(+)/PCBM(-) has been observed in this composite material. The time-domain ESE shape for different delays between the laser flash and the microwave pulse sequence has been analyzed. In order to explain the evolution of the out-of-phase ESE signal as a function of the delay between the microwave pulses, a model of the CT state is proposed. The hole is assumed to be delocalized on the P3HT chain over several thiophene subunits, while the point-dipole approximation is used to describe the interaction with the electron on PCBM. The distribution of distances between the positive and negative charges in the CT state has been evaluated.
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Total citations:
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GOST
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Lukina E. A. et al. Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite // Journal of Physical Chemistry B. 2015. Vol. 119. No. 43. pp. 13543-13548.
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Lukina E. A., Popov A. A., Uvarov M. N., Kulik L. V. Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite // Journal of Physical Chemistry B. 2015. Vol. 119. No. 43. pp. 13543-13548.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.jpcb.5b02142
UR - https://doi.org/10.1021/acs.jpcb.5b02142
TI - Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite
T2 - Journal of Physical Chemistry B
AU - Lukina, Ekaterina A
AU - Popov, A. A.
AU - Uvarov, Mikhail N.
AU - Kulik, Leonid V.
PY - 2015
DA - 2015/04/22
PB - American Chemical Society (ACS)
SP - 13543-13548
IS - 43
VL - 119
PMID - 25867974
SN - 1520-6106
SN - 1520-5207
SN - 1089-5647
ER -
Cite this
BibTex (up to 50 authors)
Copy
@article{2015_Lukina,
author = {Ekaterina A Lukina and A. A. Popov and Mikhail N. Uvarov and Leonid V. Kulik},
title = {Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite},
journal = {Journal of Physical Chemistry B},
year = {2015},
volume = {119},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acs.jpcb.5b02142},
number = {43},
pages = {13543--13548},
doi = {10.1021/acs.jpcb.5b02142}
}
Cite this
MLA
Copy
Lukina, Ekaterina A., et al. “Out-of-Phase Electron Spin Echo Studies of Light-Induced Charge-Transfer States in P3HT/PCBM Composite.” Journal of Physical Chemistry B, vol. 119, no. 43, Apr. 2015, pp. 13543-13548. https://doi.org/10.1021/acs.jpcb.5b02142.