Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide
Ryoichi Tatara
1
,
David G. Kwabi
2
,
Thomas Batcho
2
,
M. Tulodziecki
2
,
Kenta Watanabe
1
,
Hoi-min Kwon
1
,
Morgan L. Thomas
1
,
Kazuhide Ueno
1
,
Carl V. Thompson
2
,
Kaoru Dokko
1
,
Yang Shao-Horn
2
,
Publication type: Journal Article
Publication date: 2017-04-20
scimago Q1
wos Q3
SJR: 0.914
CiteScore: 6.2
Impact factor: 3.2
ISSN: 19327447, 19327455
Surfaces, Coatings and Films
Electronic, Optical and Magnetic Materials
Physical and Theoretical Chemistry
General Energy
Abstract
The performance of current Li–air batteries is greatly limited by critical obstacles such as electrolyte decomposition, high charging overpotentials, and limited cycle life. Thus, much effort is devoted to fundamental studies to understand the mechanisms of discharge/charge processes and overcome the above-mentioned obstacles. In particular, the search for new stable electrolytes is vital for long-lasting and highly cyclable batteries. The highly reactive lithium superoxide intermediate (LiO2) produced during discharge process can react with the electrolyte and produce a variety of byproducts that will shorten battery life span. To study this degradation mechanism, we investigated oxygen reduction reaction (ORR) in highly concentrated electrolyte solutions of lithium bis(trifluoromethanesulfonyl)amide (Li[TFSA])/dimethyl sulfoxide (DMSO). On the basis of rotating ring disk electrode measurements, we showed that LiO2 dissolution can be limited by increasing lithium salt concentration over 2.3 mol dm–3. Our...
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87
Total citations:
87
Citations from 2024:
19
(21%)
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GOST
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Tatara R. et al. Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide // Journal of Physical Chemistry C. 2017. Vol. 121. No. 17. pp. 9162-9172.
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Tatara R., Kwabi D. G., Batcho T., Tulodziecki M., Watanabe K., Kwon H., Thomas M. L., Ueno K., Thompson C. V., Dokko K., Shao-Horn Y., Watanabe M. Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide // Journal of Physical Chemistry C. 2017. Vol. 121. No. 17. pp. 9162-9172.
Cite this
RIS
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TY - JOUR
DO - 10.1021/acs.jpcc.7b01738
UR - https://doi.org/10.1021/acs.jpcc.7b01738
TI - Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide
T2 - Journal of Physical Chemistry C
AU - Tatara, Ryoichi
AU - Kwabi, David G.
AU - Batcho, Thomas
AU - Tulodziecki, M.
AU - Watanabe, Kenta
AU - Kwon, Hoi-min
AU - Thomas, Morgan L.
AU - Ueno, Kazuhide
AU - Thompson, Carl V.
AU - Dokko, Kaoru
AU - Shao-Horn, Yang
AU - Watanabe, Masayoshi
PY - 2017
DA - 2017/04/20
PB - American Chemical Society (ACS)
SP - 9162-9172
IS - 17
VL - 121
SN - 1932-7447
SN - 1932-7455
ER -
Cite this
BibTex (up to 50 authors)
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@article{2017_Tatara,
author = {Ryoichi Tatara and David G. Kwabi and Thomas Batcho and M. Tulodziecki and Kenta Watanabe and Hoi-min Kwon and Morgan L. Thomas and Kazuhide Ueno and Carl V. Thompson and Kaoru Dokko and Yang Shao-Horn and Masayoshi Watanabe},
title = {Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide},
journal = {Journal of Physical Chemistry C},
year = {2017},
volume = {121},
publisher = {American Chemical Society (ACS)},
month = {apr},
url = {https://doi.org/10.1021/acs.jpcc.7b01738},
number = {17},
pages = {9162--9172},
doi = {10.1021/acs.jpcc.7b01738}
}
Cite this
MLA
Copy
Tatara, Ryoichi, et al. “Oxygen Reduction Reaction in Highly Concentrated Electrolyte Solutions of Lithium Bis(trifluoromethanesulfonyl)amide/Dimethyl Sulfoxide.” Journal of Physical Chemistry C, vol. 121, no. 17, Apr. 2017, pp. 9162-9172. https://doi.org/10.1021/acs.jpcc.7b01738.